Age-dating of highly enriched Uranium by γ-spectrometry

被引:19
作者
Nguyen, CT [1 ]
机构
[1] Hungarian Acad Sci, Inst Isotopes, H-1525 Budapest, Hungary
关键词
uranium age dating; low background gamma-spectrometry; nuclear forensics; illicit trafficking of nuclear materials; fissile material cut-off treaty;
D O I
10.1016/j.nimb.2004.10.089
中图分类号
TH7 [仪器、仪表];
学科分类号
0804 ; 080401 ; 081102 ;
摘要
A non-destructive, gamma-spectrometric method for uranium age-dating is reported for the first time. The method relies on measuring the daughter/parent activity ratio Bi-214/U-234 by low-background, high-resolution gamma-spectrometry and does not require the use of reference samples of known ages. The initial methodology was derived during a "Round-Robin" exercise, in which the properties of a HEU material relevant to nuclear forensics were assessed by several laboratories. The Uranium-age obtained by this gamma-spectrometric method is in agreement with the results reported by other participating laboratories, which used mass-spectrometry for age dating. (C) 2004 Elsevier B.V. All rights reserved.
引用
收藏
页码:103 / 110
页数:8
相关论文
共 16 条
  • [1] Assessment of the Pu content of Pu-Be neutron sources
    Bagi, J
    Nguyen, TC
    Lakosi, L
    [J]. NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 2004, 222 (1-2) : 242 - 248
  • [2] BERLIZOV AN, IAEASM3671405P
  • [3] Browne E., 1986, Table of Radioactive Isotopes
  • [4] CLARK D, 1996, UCRLID125727
  • [5] DUDDER GB, 2002, 7 M INT TECHN WORK G
  • [6] GUNNINK R, 1990, UCRLLR103220, V1
  • [7] Gunnink R., 1994, UCRLJC114713
  • [8] KOCHEROV N, 1997, INDCNDS376 IAEA
  • [9] *MGA, SOFTW US MAN SOFTW V
  • [10] Age determination of highly enriched uranium:: Separation and analysis of 231Pa
    Morgenstern, A
    Apostolidis, C
    Mayer, K
    [J]. ANALYTICAL CHEMISTRY, 2002, 74 (21) : 5513 - 5516