ACTIVE BROWNIAN PARTICLES;
DENSITY-FUNCTIONAL THEORY;
SEPARATION;
FLUIDS;
DISKS;
D O I:
10.1103/PhysRevLett.117.208003
中图分类号:
O4 [物理学];
学科分类号:
0702 ;
摘要:
We develop a general theory for describing phase coexistence between nonequilibrium steady states in Brownian systems, based on power functional theory [M. Schmidt and J. M. Brader, J. Chem. Phys. 138, 214101 (2013)]. We apply the framework to the special case of fluid-fluid phase separation of active soft sphere swimmers. The central object of the theory, the dissipated free power, is calculated via computer simulations and compared to a simple analytical approximation. The theory describes well the simulation data and predicts motility-induced phase separation due to avoidance of dissipative clusters.