Nonequilibrium Phase Behavior from Minimization of Free Power Dissipation

被引:29
作者
Krinninger, Philip [1 ]
Schmidt, Matthias [1 ]
Brader, Joseph M. [2 ]
机构
[1] Univ Bayreuth, Inst Phys, Theoret Phys 2, D-95440 Bayreuth, Germany
[2] Univ Fribourg, Soft Matter Theory, CH-1700 Fribourg, Switzerland
关键词
ACTIVE BROWNIAN PARTICLES; DENSITY-FUNCTIONAL THEORY; SEPARATION; FLUIDS; DISKS;
D O I
10.1103/PhysRevLett.117.208003
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We develop a general theory for describing phase coexistence between nonequilibrium steady states in Brownian systems, based on power functional theory [M. Schmidt and J. M. Brader, J. Chem. Phys. 138, 214101 (2013)]. We apply the framework to the special case of fluid-fluid phase separation of active soft sphere swimmers. The central object of the theory, the dissipated free power, is calculated via computer simulations and compared to a simple analytical approximation. The theory describes well the simulation data and predicts motility-induced phase separation due to avoidance of dissipative clusters.
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收藏
页数:5
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