Superlinear emission in bare perovskite: amplified spontaneous emission in disordered film versus single crystal lasing

被引:1
作者
Biccari, F. [1 ]
Gabelloni, F. [1 ]
Francioni, C. [1 ]
La China, F. [1 ]
Caselli, N. [1 ]
Intonti, F. [1 ]
Gurioli, M. [1 ]
Lee, J. [2 ]
Leblebici, S. [2 ]
Weber-Bargioni, A. [2 ]
Vinattieri, A. [1 ]
机构
[1] Univ Florence, LENS, Dept Phys & Astron, I-50019 Sesto Fiorentino, Italy
[2] Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA USA
关键词
perovskites; microphotoluminescence; near field spectroscopuy; lasing; SOLAR-CELLS; HALIDE PEROVSKITES; LIGHT;
D O I
10.1016/j.matpr.2017.05.005
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We present an experimental study concerning the superlinear emission in organic-inorganic halide perovskites. Microphotoluminescence experiments under CW and picosecond excitation condition at low temperature and near field optical photoluminescence spectra at room temperature provide clear evidence of the very different origin of the superlinear regime in disordered films and microplates/microwires. Insights on the origin of modal structures of the emission spectra in the high excitation regime will be given by polarization-resolved photoluminescence experiments. (C) 2017 Elsevier Ltd.
引用
收藏
页码:S12 / S18
页数:7
相关论文
共 9 条
  • [1] Random lasing in organo-lead halide perovskite microcrystal networks
    Dhanker, R.
    Brigeman, A. N.
    Larsen, A. V.
    Stewart, R. J.
    Asbury, J. B.
    Giebink, N. C.
    [J]. APPLIED PHYSICS LETTERS, 2014, 105 (15)
  • [2] The light and shade of perovskite solar cells
    Graetzel, Michael
    [J]. NATURE MATERIALS, 2014, 13 (09) : 838 - 842
  • [3] Perovskite-Based Solar Cells
    Hodes, Gary
    [J]. SCIENCE, 2013, 342 (6156) : 317 - 318
  • [4] Efficient Hybrid Solar Cells Based on Meso-Superstructured Organometal Halide Perovskites
    Lee, Michael M.
    Teuscher, Joel
    Miyasaka, Tsutomu
    Murakami, Takurou N.
    Snaith, Henry J.
    [J]. SCIENCE, 2012, 338 (6107) : 643 - 647
  • [5] Stranks SD, 2015, NAT NANOTECHNOL, V10, P391, DOI [10.1038/nnano.2015.90, 10.1038/NNANO.2015.90]
  • [6] Sutherland BR, 2016, NAT PHOTONICS, V10, P295, DOI [10.1038/nphoton.2016.62, 10.1038/NPHOTON.2016.62]
  • [7] Charge carrier recombination channels in the low-temperature phase of organic-inorganic lead halide perovskite thin films
    Wehrenfennig, Christian
    Liu, Mingzhen
    Snaith, Henry J.
    Johnston, Michael B.
    Herz, Laura M.
    [J]. APL MATERIALS, 2014, 2 (08):
  • [8] Xing GC, 2014, NAT MATER, V13, P476, DOI [10.1038/nmat3911, 10.1038/NMAT3911]
  • [9] Zhu HM, 2015, NAT MATER, V14, P636, DOI [10.1038/nmat4271, 10.1038/NMAT4271]