Specific-heat evidence for octupolar ordering in SmRU4P12

被引:34
作者
Aoki, Yuji [1 ]
Sanada, Shotaro [1 ]
Kikuchi, Daisuke [1 ]
Sugawara, Hitoshi [1 ]
Sato, Hideyuki [1 ]
机构
[1] Tokyo Metropolitan Univ, Dept Phys, Tokyo 1920397, Japan
关键词
filled skutterudite; SmRU4P12; octupole ordering; nuclear specific heat;
D O I
10.1143/JPSJ.76.113703
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We measured specific heat in the anomalous ordered phase (T < 16.5K) of filled skutterudite SmRU4P12. From the hyperfine-enhanced Sm nuclear contribution, the ordered Sm dipole moment has been accurately determined to be 0.29 +/- 0.01 mu(B), which is strongly reduced for usual dipolar ordering. We demonstrate that this finding along with other physical quantities provide strong evidence that the primary order parameter is Gamma(4u)-type octupole. The ordered state provides the first example of an octupolar ordering accompanied by nonzero parasitic dipole moments.
引用
收藏
页数:4
相关论文
共 30 条
[1]   Anomalous heavy-fermion and ordered states in the filled skutterudite PrFe4P12 -: art. no. 064446 [J].
Aoki, Y ;
Namiki, T ;
Matsuda, TD ;
Abe, K ;
Sugawara, H ;
Sato, H .
PHYSICAL REVIEW B, 2002, 65 (06) :1-7
[2]   HYPERFINE INTERACTIONS IN RARE-EARTH METALS [J].
BLEANEY, B .
JOURNAL OF APPLIED PHYSICS, 1963, 34 (04) :1024-&
[3]   Evidence for magnetic ordering associated with metal-insulator transition in SmRu4P12 studied by muon spin relaxation [J].
Hachitani, K ;
Fukazawa, H ;
Kohori, Y ;
Watanabe, I ;
Sekine, C ;
Shirotani, I .
PHYSICAL REVIEW B, 2006, 73 (05)
[4]   Appearance of successive phase transition in SmRU4P12 under high magnetic fields probed by 31P nuclear magnetic resonance [J].
Hachitani, Kenichi ;
Amanuma, Hideaki ;
Fukazawa, Hideto ;
Kohori, Yoh ;
Koyama, Keiichi ;
Kumagai, Ken-ichi ;
Sekine, Chihiro ;
Shirotani, Ichimin .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2006, 75 (12)
[5]   Conduction bands in the filled skutterudites [J].
Harima, H ;
Takegahara, K .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2003, 15 (28) :S2081-S2086
[6]   Multipole fluctuations in filled skutterudites [J].
Hotta, T .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2005, 74 (09) :2425-2429
[7]   Multipole susceptibility of multiorbital Anderson model coupled with Jahn-Teller phonons [J].
Hotta, Takashi .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2007, 76 (03)
[8]   Evolution of local magnetic state in SmRu4P12 probed by muon spin relaxation [J].
Ito, Takashi U. ;
Higemoto, Wataru ;
Ohishi, Kazuki ;
Fujimoto, Tatsuya ;
Heffner, Robert H. ;
Nishida, Nobuhiko ;
Satoh, Kazuhiko ;
Sugawara, Hitoshi ;
Aoki, Yuji ;
Kikuchi, Daisuke ;
Sato, Hideyuki .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2007, 76 (05)
[9]   Evolution of 4f electron states in the metal-insulator transition of PrRu4P12 -: art. no. 024414 [J].
Iwasa, K ;
Hao, LJ ;
Kuwahara, K ;
Kohgi, M ;
Saha, SR ;
Sugawara, H ;
Aoki, Y ;
Sato, H ;
Tayama, T ;
Sakakibara, T .
PHYSICAL REVIEW B, 2005, 72 (02)
[10]   Microscopic theory of multipole ordering in NpO2 -: art. no. 140404 [J].
Kubo, K ;
Hotta, T .
PHYSICAL REVIEW B, 2005, 71 (14)