Pollution by nitrogen oxides:: an approach to NOx abatement by using sorbing catalytic materials

被引:224
作者
Gómez-García, MA [1 ]
Pitchon, V [1 ]
Kiennemann, A [1 ]
机构
[1] ULP, ECPM, CNRS,Lab Mat Surfaces & Procedes Catalyse, UMR 7515,LMSPC, F-67087 Strasbourg, France
关键词
nitrogen oxide; selective catalytic reduction; double-layered cuprate;
D O I
10.1016/j.envint.2004.09.006
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This article summarises the abatement of NO, pollution by using sorbing catalytic materials with especial relevance to the challenge presented in fixed installations sources. A general vision of the origins of the different pollutants, with emphasis on nitrogen oxides formation, is presented as introduction. The impact of NO, pollution comprises additionally a quick view of its toxicity and environmental effects. Actual solutions are presented especially the case of the selective catalytic reduction (SCR) process with its advantages and difficulties. The new concepts for NOx abatement are also analysed. In such a way, updated information on solid sorbents for NOx removal is provided by including metal oxides, spinelles, perovskites, double-layered cuprates, zeolites, carbonaceous materials, heteropolyacids (HPAs), and supported heteropolyacids. The possibility of reducing those sorbed NOx is also underlined. Sorption mechanisms are analysed and clarified by emphasising convergence and disagreement points. (c) 2004 Elsevier Ltd. All rights reserved.
引用
收藏
页码:445 / 467
页数:23
相关论文
共 150 条
[1]   Dissociative adsorption of NO on TiO2(110) argon ion bombarded surfaces [J].
Abad, J ;
Böhme, O ;
Román, E .
SURFACE SCIENCE, 2004, 549 (02) :134-142
[2]   COADSORPTION OF NITROGEN MONOXIDE AND NITROGEN-DIOXIDE IN ZEOLITIC DE-NOX CATALYSTS [J].
ADELMAN, BJ ;
LEI, GD ;
SACHTLER, WMH .
CATALYSIS LETTERS, 1994, 28 (2-4) :119-130
[3]   KINETIC AND INFRARED SPECTROSCOPIC STUDIES OF FE-Y ZEOLITES FOR THE SELECTIVE CATALYTIC REDUCTION OF NITRIC-OXIDE BY AMMONIA [J].
AMIRIDIS, MD ;
PUGLISI, F ;
DUMESIC, JA ;
MILLMAN, WS ;
TOPSOE, NY .
JOURNAL OF CATALYSIS, 1993, 142 (02) :572-584
[4]   Selective catalytic reduction of nitric oxide by hydrocarbons [J].
Amiridis, MD ;
Zhang, TJ ;
Farrauto, RJ .
APPLIED CATALYSIS B-ENVIRONMENTAL, 1996, 10 (1-3) :203-227
[5]   REMOVAL OF NOX THROUGH SORPTION-DESORPTION CYCLES OVER METAL-OXIDES AND ZEOLITES [J].
ARAI, H ;
MACHIDA, M .
CATALYSIS TODAY, 1994, 22 (01) :97-109
[6]   Catalytic solutions to reduce pollutants [J].
Armor, JN .
CATALYSIS TODAY, 1997, 38 (02) :163-167
[7]   NOx/hydrocarbon reactions over gallium loaded zeolites: A review [J].
Armor, JN .
CATALYSIS TODAY, 1996, 31 (3-4) :191-198
[8]   HETEROPOLYACIDS AND THEIR SALTS SUPPORTED ON ACIDIC ION-EXCHANGE RESIN AS HIGHLY-ACTIVE SOLID-ACID CATALYSTS [J].
BABA, T ;
ONO, Y .
APPLIED CATALYSIS, 1986, 22 (02) :321-324
[9]   Computer simulation studies of bulk reduction and oxygen migration in CeO2-ZrO2 solid solutions [J].
Balducci, G ;
Kaspar, J ;
Fornasiero, P ;
Graziani, M ;
Islam, MS ;
Gale, JD .
JOURNAL OF PHYSICAL CHEMISTRY B, 1997, 101 (10) :1750-1753
[10]   Surface and reduction energetics of the CeO2-ZrO2 catalysts [J].
Balducci, G ;
Kaspar, J ;
Fornasiero, P ;
Graziani, M ;
Islam, MS .
JOURNAL OF PHYSICAL CHEMISTRY B, 1998, 102 (03) :557-561