Fluoride removal from water by granular ceramic adsorption

被引：135

作者：

Chen, Nan ^{[1
,2
]}

Zhang, Zhenya ^{[1
]}

Feng, Chuanping ^{[2
]}

Sugiura, Norio ^{[1
]}

Li, Miao ^{[1
,2
]}

Chen, Rongzhi ^{[1
]}

机构：

[1] Univ Tsukuba, Grad Sch Life & Environm Sci, Tsukuba, Ibaraki 3058572, Japan

[2] China Univ Geosci Beijing, Sch Water Resources & Environm, Beijing 100083, Peoples R China

来源：

JOURNAL OF COLLOID AND INTERFACE SCIENCE | 2010年 / 348卷 / 02期

关键词：

Granular ceramic; Fluoride removal; Adsorption isotherms; Adsorption kinetics; AQUEOUS-SOLUTION; DRINKING-WATER; DEFLUORIDATION; SORPTION; EFFLUENT; IONS;

D O I：

10.1016/j.jcis.2010.04.048

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

A new medium, granular ceramic, has been developed for fluoride removal from water. Granular ceramic is a solid-phase medium that produces a stable Al-Fe surface complex for fluoride adsorption. BET, SEM, and EDS were used to characterize the physical attributes (particle size, pore size and distribution, surface roughness) of the granular ceramic. Fluoride adsorption characteristics were studied in a batch system with respect to changes in initial concentration of fluoride, pH of solution, and coexisting ions. Fluoride adsorption was found to be pH dependent and the maximum removal of fluoride was obtained at pH 5.0-8.0. equilibrium adsorption data were obtained at 293, 303, and 323 K, and interpreted in terms of the Langmuir and Freundlich isotherm equations. The experimental data revealed that the Freundlich isotherm equation gives a more satisfactory fit for fluoride removal. The adsorption process was observed to follow a pseudo-second-order kinetic model and intraparticle diffusion was indicated to play a major role in fluoride uptake. Fluoride adsorption was reduced in the presence of phosphate and sulfate ions and increased slightly in the presence of chloride and nitrate ions. (C) 2010 Elsevier Inc. All rights reserved.

引用

页码：579 / 584

页数：6

共 35 条

[1]

[Anonymous], 2002, WATER WASTEWATER MON, V4, P193

[2]

[Anonymous], 2006, WORLD HLTH ORG, DOI DOI 10.5942/JAWWA.2017.109.0087

[3] Investigations on the kinetics and mechanisms of sorptive removal of fluoride from water using alumina cement granules [J].

Ayoob, S. ;

Gupta, A. K. ;

Bhakat, P. B. ;

Bhat, Venugopal T. .

CHEMICAL ENGINEERING JOURNAL, 2008, 140 (1-3) :6-14

[4] Adsorption of fluoride from aqueous solution by a synthetic Iron(III)-Aluminum(III) mixed oxide [J].

Biswas, Krishna ;

Saha, Sanat Kumar ;

Ghosh, Uday Chand .

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2007, 46 (16) :5346-5356

[5] DEFLUORIDATION OF WATER BY ADSORPTION ON FLY-ASH [J].

CHATURVEDI, AK ;

YADAVA, KP ;

PATHAK, KC ;

SINGH, VN .

WATER AIR AND SOIL POLLUTION, 1990, 49 (1-2) :51-61

[6] Adsorption of fluoride, chloride, bromide, and bromate ions on a novel ion exchanger [J].

Chubar, NI ;

Samanidou, VF ;

Kouts, VS ;

Gallios, GG ;

Kanibolotsky, VA ;

Strelko, VV ;

Zhuravlev, IZ .

JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2005, 291 (01) :67-74

[7] The cause of endemic fluorosis in western Guizhou Province, Southwest China [J].

Dai, SF ;

Ren, DY ;

Ma, SM .

FUEL, 2004, 83 (14-15) :2095-2098

[8] Pseudo-second order model for sorption processes [J].

Ho, YS ;

McKay, G .

PROCESS BIOCHEMISTRY, 1999, 34 (05) :451-465

[9] Removal of fluoride from semiconductor wastewater by electrocoagulation-flotation [J].

Hu, CY ;

Lo, SL ;

Kuan, WH ;

Lee, YD .

WATER RESEARCH, 2005, 39 (05) :895-901

[10]

Lagergren SK., 1898, KUNGLIGA SVENSKA VET, V24, P1, DOI DOI 10.1007/BF01501332

← 1 2 3 4 →