Dechlorane Plus (DP) in air and plants at an electronic waste (e-waste) site in South China

被引:92
作者
Chen, She-Jun [1 ]
Tian, Mi [1 ,2 ]
Wang, Jing [1 ,2 ]
Shi, Tian [1 ,2 ]
Luo, Yong [3 ]
Luo, Xiao-Jun [1 ]
Mai, Bi-Xian [1 ]
机构
[1] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
[2] Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China
[3] Guangdong Forestry Survey & Planning Inst, Guangzhou 510520, Guangdong, Peoples R China
基金
美国国家科学基金会;
关键词
Dechlorane Plus (DP); Air and plant; E-waste; Temporal distribution; Dechlorination; BROMINATED FLAME RETARDANTS; POLYCYCLIC AROMATIC-HYDROCARBONS; POLYBROMINATED DIPHENYL ETHERS; SEMIVOLATILE ORGANIC-COMPOUNDS; GREAT-LAKES; POLYCHLORINATED-BIPHENYLS; ORGANOCHLORINE COMPOUNDS; TREE BARK; LEAF-AREA; ENVIRONMENT;
D O I
10.1016/j.envpol.2011.01.026
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Air and foliage samples (Eucalyptus spp. and Pinus massoniana Lamb.) were collected from e-waste and reference sites in South China and analyzed for Dechlorane Plus (DP) and two dechlorinated DPs. DP concentrations in the air were 13.1-1794 pg/m(3) for the e-waste site and 0.47-35.7 pg/m(3) for the reference site, suggesting the recycling of e-waste is an important source of DP to the environment. Plant DP, with concentrations of 0.45-51.9 ng/g dry weight at the e-waste site and 0.09-2.46 ng/g at the reference site, exhibited temporal patterns similar to the air DP except for pine needle at the reference site. The air-plant exchange of DP could be described with the two-compartment model. Anti-Cl(11) DP was measured in most air and plant samples from the e-waste site. The ratios of anti-Cl(11) DP to anti-DP in the air and plants may indicate the preferential uptake of dechlorinated DP by plant compared with DP. (C) 2011 Elsevier Ltd. All rights reserved.
引用
收藏
页码:1290 / 1296
页数:7
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