Dechlorane Plus (DP) in air and plants at an electronic waste (e-waste) site in South China

被引:92
作者
Chen, She-Jun [1 ]
Tian, Mi [1 ,2 ]
Wang, Jing [1 ,2 ]
Shi, Tian [1 ,2 ]
Luo, Yong [3 ]
Luo, Xiao-Jun [1 ]
Mai, Bi-Xian [1 ]
机构
[1] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
[2] Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China
[3] Guangdong Forestry Survey & Planning Inst, Guangzhou 510520, Guangdong, Peoples R China
基金
美国国家科学基金会;
关键词
Dechlorane Plus (DP); Air and plant; E-waste; Temporal distribution; Dechlorination; BROMINATED FLAME RETARDANTS; POLYCYCLIC AROMATIC-HYDROCARBONS; POLYBROMINATED DIPHENYL ETHERS; SEMIVOLATILE ORGANIC-COMPOUNDS; GREAT-LAKES; POLYCHLORINATED-BIPHENYLS; ORGANOCHLORINE COMPOUNDS; TREE BARK; LEAF-AREA; ENVIRONMENT;
D O I
10.1016/j.envpol.2011.01.026
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Air and foliage samples (Eucalyptus spp. and Pinus massoniana Lamb.) were collected from e-waste and reference sites in South China and analyzed for Dechlorane Plus (DP) and two dechlorinated DPs. DP concentrations in the air were 13.1-1794 pg/m(3) for the e-waste site and 0.47-35.7 pg/m(3) for the reference site, suggesting the recycling of e-waste is an important source of DP to the environment. Plant DP, with concentrations of 0.45-51.9 ng/g dry weight at the e-waste site and 0.09-2.46 ng/g at the reference site, exhibited temporal patterns similar to the air DP except for pine needle at the reference site. The air-plant exchange of DP could be described with the two-compartment model. Anti-Cl(11) DP was measured in most air and plant samples from the e-waste site. The ratios of anti-Cl(11) DP to anti-DP in the air and plants may indicate the preferential uptake of dechlorinated DP by plant compared with DP. (C) 2011 Elsevier Ltd. All rights reserved.
引用
收藏
页码:1290 / 1296
页数:7
相关论文
共 38 条
  • [1] General formulation of characteristic travel distance for semivolatile organic chemicals in a multimedia environment
    Bennett, DH
    McKone, TE
    Matthies, M
    Kastenberg, WE
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1998, 32 (24) : 4023 - 4030
  • [3] An overview of brominated flame retardants in the environment
    de Wit, CA
    [J]. CHEMOSPHERE, 2002, 46 (05) : 583 - 624
  • [4] Single leaf area estimation models based on leaf weight of eucalyptus in southern China
    Diao J.
    Lei X.-D.
    Hong L.-X.
    Rong J.-T.
    Shi Q.
    [J]. Journal of Forestry Research, 2010, 21 (1) : 73 - 76
  • [5] Air-surface exchange of polybrominated biphenyl ethers and polychlorinated biphenyls
    Gouin, T
    Thomas, GO
    Cousins, I
    Barber, J
    Mackay, D
    Jones, KC
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2002, 36 (07) : 1426 - 1434
  • [6] UPTAKE OF GASEOUS DDE IN SPRUCE NEEDLES
    HAUK, H
    UMLAUF, G
    MCLACHLAN, MS
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1994, 28 (13) : 2372 - 2379
  • [7] Dechlorane plus, a chlorinated flame retardant, in the Great Lakes
    Hoh, E
    Zhu, LY
    Hites, RA
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2006, 40 (04) : 1184 - 1189
  • [8] Atmospheric deposition of semivolatile organic compounds to two forest canopies
    Horstmann, M
    McLachlan, MS
    [J]. ATMOSPHERIC ENVIRONMENT, 1998, 32 (10) : 1799 - 1809
  • [9] Grass-air exchange of polychlorinated biphenyls
    Hung, H
    Thomas, GO
    Jones, KC
    Mackay, D
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2001, 35 (20) : 4066 - 4073
  • [10] PCBs and selected organochlorine compounds in Italian mountain air: the influence of altitude and forest ecosystem type
    Jaward, FM
    Di Guardo, A
    Nizzetto, L
    Cassani, C
    Raffaele, F
    Ferretti, R
    Jones, KC
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2005, 39 (10) : 3455 - 3463