Dechlorane Plus (DP) in air and plants at an electronic waste (e-waste) site in South China

被引:91
作者
Chen, She-Jun [1 ]
Tian, Mi [1 ,2 ]
Wang, Jing [1 ,2 ]
Shi, Tian [1 ,2 ]
Luo, Yong [3 ]
Luo, Xiao-Jun [1 ]
Mai, Bi-Xian [1 ]
机构
[1] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
[2] Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China
[3] Guangdong Forestry Survey & Planning Inst, Guangzhou 510520, Guangdong, Peoples R China
基金
美国国家科学基金会;
关键词
Dechlorane Plus (DP); Air and plant; E-waste; Temporal distribution; Dechlorination; BROMINATED FLAME RETARDANTS; POLYCYCLIC AROMATIC-HYDROCARBONS; POLYBROMINATED DIPHENYL ETHERS; SEMIVOLATILE ORGANIC-COMPOUNDS; GREAT-LAKES; POLYCHLORINATED-BIPHENYLS; ORGANOCHLORINE COMPOUNDS; TREE BARK; LEAF-AREA; ENVIRONMENT;
D O I
10.1016/j.envpol.2011.01.026
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Air and foliage samples (Eucalyptus spp. and Pinus massoniana Lamb.) were collected from e-waste and reference sites in South China and analyzed for Dechlorane Plus (DP) and two dechlorinated DPs. DP concentrations in the air were 13.1-1794 pg/m(3) for the e-waste site and 0.47-35.7 pg/m(3) for the reference site, suggesting the recycling of e-waste is an important source of DP to the environment. Plant DP, with concentrations of 0.45-51.9 ng/g dry weight at the e-waste site and 0.09-2.46 ng/g at the reference site, exhibited temporal patterns similar to the air DP except for pine needle at the reference site. The air-plant exchange of DP could be described with the two-compartment model. Anti-Cl(11) DP was measured in most air and plant samples from the e-waste site. The ratios of anti-Cl(11) DP to anti-DP in the air and plants may indicate the preferential uptake of dechlorinated DP by plant compared with DP. (C) 2011 Elsevier Ltd. All rights reserved.
引用
收藏
页码:1290 / 1296
页数:7
相关论文
共 38 条
[1]   General formulation of characteristic travel distance for semivolatile organic chemicals in a multimedia environment [J].
Bennett, DH ;
McKone, TE ;
Matthies, M ;
Kastenberg, WE .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1998, 32 (24) :4023-4030
[2]   Flame retardants are the suspected source of a new compound in the environment [J].
Betts, Kellyn .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2010, 44 (02) :546-547
[3]   An overview of brominated flame retardants in the environment [J].
de Wit, CA .
CHEMOSPHERE, 2002, 46 (05) :583-624
[4]   Single leaf area estimation models based on leaf weight of eucalyptus in southern China [J].
Diao J. ;
Lei X.-D. ;
Hong L.-X. ;
Rong J.-T. ;
Shi Q. .
Journal of Forestry Research, 2010, 21 (1) :73-76
[5]   Air-surface exchange of polybrominated biphenyl ethers and polychlorinated biphenyls [J].
Gouin, T ;
Thomas, GO ;
Cousins, I ;
Barber, J ;
Mackay, D ;
Jones, KC .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2002, 36 (07) :1426-1434
[6]   UPTAKE OF GASEOUS DDE IN SPRUCE NEEDLES [J].
HAUK, H ;
UMLAUF, G ;
MCLACHLAN, MS .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1994, 28 (13) :2372-2379
[7]   Dechlorane plus, a chlorinated flame retardant, in the Great Lakes [J].
Hoh, E ;
Zhu, LY ;
Hites, RA .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2006, 40 (04) :1184-1189
[8]   Atmospheric deposition of semivolatile organic compounds to two forest canopies [J].
Horstmann, M ;
McLachlan, MS .
ATMOSPHERIC ENVIRONMENT, 1998, 32 (10) :1799-1809
[9]   Grass-air exchange of polychlorinated biphenyls [J].
Hung, H ;
Thomas, GO ;
Jones, KC ;
Mackay, D .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2001, 35 (20) :4066-4073
[10]   PCBs and selected organochlorine compounds in Italian mountain air: the influence of altitude and forest ecosystem type [J].
Jaward, FM ;
Di Guardo, A ;
Nizzetto, L ;
Cassani, C ;
Raffaele, F ;
Ferretti, R ;
Jones, KC .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2005, 39 (10) :3455-3463