Source apportionment and seasonal variation of PM2.5 carbonaceous aerosol in the Beijing-Tianjin-Hebei Region of China

被引:110
作者
Wang, Gang [1 ,3 ]
Cheng, Shuiyuan [1 ,3 ]
Li, Jianbing [2 ]
Lang, Jianlei [1 ,3 ]
Wen, Wei [1 ,3 ]
Yang, Xiaowen [1 ,3 ]
Tian, Liang [1 ,3 ]
机构
[1] Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100022, Peoples R China
[2] Univ No British Columbia, Environm Engn Program, Prince George, BC V2N 4Z9, Canada
[3] Collaborat Innovat Ctr Elect Vehicles, Beijing 100081, Peoples R China
关键词
Carbonaceous aerosol; Elemental carbon; Organic carbon; PM2.5; Principal component analysis; SECONDARY ORGANIC AEROSOL; ELEMENTAL CARBON; CHEMICAL-COMPOSITION; DESCRIPTIVE ANALYSIS; SOURCE PROFILES; HONG-KONG; URBAN; TEMPERATURE; VISIBILITY; EMISSIONS;
D O I
10.1007/s10661-015-4288-x
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The seasonal variation of PM2.5 carbonaceous aerosol was investigated in Beijing and Tangshan cities of China. The characteristics of carbonaceous aerosol (e.g., organic carbon, OC and elemental carbon, EC) under different weather conditions and their source apportionment were also examined. The annual average PM2.5 concentration in the study area reached 95.6-197.3 mu g/m(3), showing seasonal and spatial variation. The carbonaceous materials accounted for 17.3-21.2% of the PM2.5, and they had a much higher content under haze weather condition. It was found that the PM2.5 contained more OC than EC. Principal component analysis (PCA) results indicated that the carbonaceous components came from mixed emission sources of coal combustion, vehicle exhaust, and biomass burning. In Beijing, the vehicle emission made a contribution of 63.0 % to the carbonaceous components of PM2.5 in summer, which is higher than that in Tangshan. While in Tangshan, the coal combustion made a contribution of 30.3 %, which is much higher than that in Beijing.
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页数:13
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