Pore growth in U-Mo/Al dispersion fuel

被引:15
作者
Kim, Yeon Soo [1 ]
Jeong, G. Y. [2 ]
Sohn, D. -S. [2 ]
Jamison, L. M. [1 ]
机构
[1] Argonne Natl Lab, 9700 South Cass Ave, Argonne, IL 60439 USA
[2] Ulsan Natl Inst Sci & Technol, 50 UNIST Gil, Ulsan 689798, South Korea
基金
新加坡国家研究基金会;
关键词
U-Mo/Al dispersion fuel; Pore growth; Porosity; In-pile data; Modeling; IRRADIATION BEHAVIOR; PARTICLE DISPERSION; ENHANCED DIFFUSION; AL MATRIX; MO FUEL; PRODUCT; ENERGIES; TENSION; SURFACE; ALLOY;
D O I
10.1016/j.jnucmat.2016.06.029
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
U-Mo/Al dispersion fuel is currently under development in the DOE's Material Management and Minimization program to convert HEU-fueled research reactors to LEU-fueled reactors. In some demanding conditions in high-power and high-performance reactors, large pores form in the interaction layers between the U-Mo fuel particles and the Al matrix, which pose a potential to cause fuel failure. In this study, comprehension of the formation and growth of these pores was explored. As a product, a model to predict pore growth and porosity increase was developed. The model includes three major topics: fission gas release from the U-Mo and the IL to the pores, stress evolution in the fuel meat, and the effect of amorphous IL growth. Well-characterized in-pile data from reduced-size plates were used to fit the model parameters. A data set from full-sized plates, independent and distinctively different from those used to fit the model parameters, was used to examine the accuracy of the model. The model showed fair agreement with the measured data. The model suggested that the growth of the IL has a critical effect on pore growth, as both its material properties and energetics are favorable to pore formation. Therefore, one area of the current effort, focused on suppressing IL growth, appears to be on the right track to improve the performance of this fuel. (C) 2016 Elsevier B.V. All rights reserved.
引用
收藏
页码:275 / 286
页数:12
相关论文
共 48 条
  • [1] U-Mo/Al-Si interaction: Influence of Si concentration
    Allenou, J.
    Palancher, H.
    Iltis, X.
    Cornen, M.
    Tougait, O.
    Tucoulou, R.
    Welcomme, E.
    Martin, Ph.
    Valot, C.
    Charollais, F.
    Anselmet, M. C.
    Lemoine, P.
    [J]. JOURNAL OF NUCLEAR MATERIALS, 2010, 399 (2-3) : 189 - 199
  • [2] MOLECULAR-DYNAMICS SIMULATIONS OF ALPHA-ALUMINA AND GAMMA-ALUMINA SURFACES
    BLONSKI, S
    GAROFALINI, SH
    [J]. SURFACE SCIENCE, 1993, 295 (1-2) : 263 - 274
  • [3] Booth A.H., 1957, METHOD CALCULATING F
  • [4] SOLIDS IN CONTACT
    BUCKLEY, DH
    FERRANTE, J
    PASHLEY, MD
    SMITH, JR
    [J]. MATERIALS SCIENCE AND ENGINEERING, 1986, 83 (02): : 177 - 188
  • [5] Farrell K, 2012, COMPREHENSIVE NUCLEAR MATERIALS, VOL 5: MATERIAL PERFORMANCE AND CORROSION/WASTE MATERIALS, P143
  • [6] Transmission electron microscopy characterization of irradiated U-7Mo/Al-2Si dispersion fuel
    Gan, J.
    Keiser, D. D., Jr.
    Wachs, D. M.
    Robinson, A. B.
    Miller, B. D.
    Allen, T. R.
    [J]. JOURNAL OF NUCLEAR MATERIALS, 2010, 396 (2-3) : 234 - 239
  • [7] A THEORY FOR THE ESTIMATION OF SURFACE AND INTERFACIAL ENERGIES .1. DERIVATION AND APPLICATION TO INTERFACIAL TENSION
    GIRIFALCO, LA
    GOOD, RJ
    [J]. JOURNAL OF PHYSICAL CHEMISTRY, 1957, 61 (07) : 904 - 909
  • [8] Golosov O.A., 2007, P INT M RED ENR RES
  • [9] Golosov O.A., 2009, T INT TOP M RES REAC
  • [10] Hamy J.M., 2004, T INT TOP M RES REAC