A review on energy chemistry of fast-charging anodes

被引：521

作者：

Cai, Wenlong ^{[1
]}

Yao, Yu-Xing ^{[1
]}

Zhu, Gao-Long ^{[1
,2
]}

Yan, Chong ^{[3
]}

Jiang, Li-Li ^{[1
,4
]}

He, Chuanxin ^{[2
]}

Huang, Jia-Qi ^{[3
]}

Zhang, Qiang ^{[1
]}

机构：

[1] Tsinghua Univ, Beijing Key Lab Green Chem React Engn & Technol D, Beijing 100084, Peoples R China

[2] Shenzhen Univ, Coll Chem & Chem Engn, Shenzhen Key Lab Funct Polymer, Shenzhen 518061, Peoples R China

[3] Beijing Inst Technol, Adv Res Inst Multidisciplinary Sci, Beijing 100081, Peoples R China

[4] Jilin Inst Chem Technol, Key Lab Special Funct Mat Jilin Prov Univ, Jilin 132022, Jilin, Peoples R China

来源：

CHEMICAL SOCIETY REVIEWS | 2020年 / 49卷 / 12期

基金：

中国国家自然科学基金; 北京市自然科学基金;

关键词：

LITHIUM-ION BATTERIES; SOLID-ELECTROLYTE INTERPHASE; MOLECULAR-DYNAMICS SIMULATION; LI-ION; GRAPHITE ANODE; PROPYLENE CARBONATE; CYCLE LIFE; NATURAL GRAPHITE; HIGH-POWER; GRAPHITE/ELECTROLYTE INTERFACE;

D O I：

10.1039/c9cs00728h

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

With the impetus to accelerate worldwide market adoption of electrical vehicles and afford consumer electronics with better user experience, advancing fast-charging technology is an inevitable trend. However, current high-energy lithium-ion batteries are unable to support ultrafast power input without any adverse consequences, with the capacity fade and safety concerns of the mainstream graphite-based anodes being the key technological barrier. The aim of this review is to summarise the fundamentals, challenges, and solutions to enable graphite anodes that are capable of high-rate charging. First, we explore the complicated yet intriguing graphite-electrolyte interface during intercalation based on existing theories. Second, we analyse the key dilemmas facing fast-charging graphite anodes. Finally, some promising strategies proposed during the past few years are highlighted so as to outline current trends and future perspectives in this field.

引用

页码：3806 / 3833

页数：28

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