Role of anisotropy in determining stability of electrodeposition at solid-solid interfaces

被引:23
作者
Ahmad, Zeeshan [1 ]
Viswanathan, Venkatasubramanian [1 ,2 ]
机构
[1] Carnegie Mellon Univ, Dept Mech Engn, Pittsburgh, PA 15213 USA
[2] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA
关键词
LITHIUM METAL BATTERIES; RECHARGEABLE BATTERIES; SUPERIONIC CONDUCTORS; STATE ELECTROLYSIS; ANODES; GROWTH; DEFORMATION; ELASTICITY; MECHANISMS; DIFFUSION;
D O I
10.1103/PhysRevMaterials.1.055403
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We investigate the stability of electrodeposition at solid-solid interfaces for materials exhibiting an anisotropic mechanical response. The stability of electrodeposition or resistance to the formation of dendrites is studied within a linear stability analysis. The deformation and stress equations are solved using the Stroh formalism and faithfully recover the boundary conditions at the interface. The stability parameter is used to quantify the stability of different solid-solid interfaces incorporating the full anisotropy of the elastic tensor of the two materials. Results show a high degree of variability in the stability parameter depending on the crystallographic orientation of the solids in contact, and point to opportunities for exploiting this effect in developing Li metal anodes.
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页数:9
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