Experimental study on gas diffusion dynamics in fractured coal: A better understanding of gas migration in in-situ coal seam

被引:115
作者
Liu, Ting [1 ,2 ]
Lin, Baiquan [1 ]
Fu, Xuehai [2 ]
Gao, Yabin [3 ]
Kong, Jia [1 ]
Zhao, Yang [1 ]
Song, Haoran [1 ]
机构
[1] China Univ Min & Technol, Sch Safety Engn, Xuzhou 221116, Jiangsu, Peoples R China
[2] China Univ Min & Technol, Minist Educ, Key Lab CBM Resources & Dynam Accumulat Proc, Xuzhou 221008, Jiangsu, Peoples R China
[3] Taiyuan Univ Technol, Coll Safety & Emergency Management Engn, Taiyuan 030024, Shanxi, Peoples R China
基金
中国国家自然科学基金; 中国博士后科学基金;
关键词
Gas diffusion; Scale effect; Granular coal; Fractured coal core; In-situ coal seam; DISPERSIVE DIFFUSION; PORE DIFFUSION; CARBON-DIOXIDE; POROUS-MEDIA; METHANE; DESORPTION; MODEL; PERMEABILITY; COEFFICIENT; TIME;
D O I
10.1016/j.energy.2020.117005
中图分类号
O414.1 [热力学];
学科分类号
摘要
In-situ coal seam is generally under the stress constraint condition. However, the powder coal is often adopted to study gas diffusion dynamics in the laboratory, in this case, the stress cannot be imposed on the coal sample. So the question is, can the laboratory test results with the powder coal reflect the gas diffusion behaviors in the in-situ coal seam? Does the confining stress affect the gas diffusion behaviors in fractured coal? To address these questions, in this work, we first investigated the effect of coal size on gas diffusion dynamics with powder coal and lump coal under unconstrained conditions. The results show that there exists an obvious scale effect for gas diffusion in coal, and a critical value of coal size has been found for the scale effect. When the coal particle size is smaller than the critical value, the effective diffusivity decreases with an increase of the particle size; and when the particle size is larger than the critical value, no obvious change can be found in the effective diffusivity. The critical value for gas diffusion corresponds to the size of the coal matrix. The essential reason for the existence of the scale effect is the differences among the pore structures of coals with various sizes. Based on the research results under the unconstrained conditions, a coal core was selected to study the effect of confining stress and pore pressure on gas diffusion under constraint condition. The results indicated that the confining stress and pore pressure have significant impact on gas diffusion in fractured coal. With an increase of the confining stress and a decrease of the pore pressure, the effective diffusivity reduces gradually. Therefore, to get an accurate understanding of the gas diffusion behavior in in-situ coal seam, during the test in the lab, both the scale effect and confining stress should be considered. The research results obtained in this work have important guiding significance to reveal gas migration in in-situ coal seams during CBM depletion, CO2-ECBM and geological sequestration of CO2. (C) 2020 Elsevier Ltd. All rights reserved.
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页数:10
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共 36 条
  • [1] Methane and carbon dioxide adsorption-diffusion experiments on coal: upscaling and modeling
    Busch, A
    Gensterblum, Y
    Krooss, BM
    Littke, R
    [J]. INTERNATIONAL JOURNAL OF COAL GEOLOGY, 2004, 60 (2-4) : 151 - 168
  • [2] Representative elementary volume estimation for porosity, moisture saturation, and air-water interfacial areas in unsaturated porous media: Data quality implications
    Costanza-Robinson, Molly S.
    Estabrook, Benjamin D.
    Fouhey, David F.
    [J]. WATER RESOURCES RESEARCH, 2011, 47
  • [3] Characteristics of methane desorption and diffusion in coal within a negative pressure environment
    Du, Yunfei
    Chen, Xiangjun
    Li, Liyang
    Wang, Peng
    [J]. FUEL, 2018, 217 : 111 - 121
  • [4] Thermo-hydro-mechanical-chemical couplings controlling CH4 production and CO2 sequestration in enhanced coalbed methane recovery
    Fan, Chaojun
    Elsworth, Derek
    Li, Sheng
    Zhou, Lijun
    Yang, Zhenhua
    Song, Yu
    [J]. ENERGY, 2019, 173 : 1054 - 1077
  • [5] Experimental simulation of replacing and displacing CH4 by injecting supercritical CO2 and its geological significance
    Fang, Huihuang
    Sang, Shuxun
    Liu, Shiqi
    Liu, Shupei
    [J]. INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL, 2019, 81 : 115 - 125
  • [6] CO2-ECBM: A Review of its Status and Global Potential
    Godec, Michael
    Koperna, George
    Gale, John
    [J]. 12TH INTERNATIONAL CONFERENCE ON GREENHOUSE GAS CONTROL TECHNOLOGIES, GHGT-12, 2014, 63 : 5858 - 5869
  • [7] Effect of moisture on the desorption and unsteady-state diffusion properties of gas in low-rank coal
    Guo, Haijun
    Yuan, Liang
    Cheng, Yuanping
    Wang, Kai
    Xu, Chao
    Zhou, Aitao
    Zang, Jie
    Liu, Jiajia
    [J]. JOURNAL OF NATURAL GAS SCIENCE AND ENGINEERING, 2018, 57 : 45 - 51
  • [8] Effects of Organic Micromolecules in coal on its Pore Structure and Gas Diffusion Characteristics
    Ji, Huaijun
    Li, Zenghua
    Yang, Yongliang
    Hu, Shaobin
    Peng, Yingjian
    [J]. TRANSPORT IN POROUS MEDIA, 2015, 107 (02) : 419 - 433
  • [9] Numerical modeling and experimental validation of anomalous time and space subdiffusion for gas transport in porous coal matrix
    Kang, Jianhong
    Zhou, Fubao
    Xia, Tongqiang
    Ye, Gaobang
    [J]. INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER, 2016, 100 : 747 - 757
  • [10] Effect of maceral composition and coal rank on gas diffusion in Australian coals
    Keshavarz, Alireza
    Sakurovs, Richard
    Grigore, Mihaela
    Sayyafzadeh, Mohammad
    [J]. INTERNATIONAL JOURNAL OF COAL GEOLOGY, 2017, 173 : 65 - 75