Probing electronic and vibrational dynamics in molecules by time-resolved photoelectron, Auger-electron, and X-ray photon scattering spectroscopy

被引：22

作者：

Bennett, Kochise ^{[1
]}

Kowalewski, Markus ^{[1
]}

Mukamel, Shaul ^{[1
]}

机构：

[1] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA

来源：

FARADAY DISCUSSIONS | 2015年 / 177卷

基金：

美国国家卫生研究院; 美国国家科学基金会;

关键词：

NONADIABATIC DYNAMICS; SPECTRA; TRANSITION; PROGRAM; URACIL;

D O I：

10.1039/c4fd00178h

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We present a unified description for time-resolved electron and photon scattering spectroscopies from molecules prepared in nonstationary states. Signals are expressed in terms of superoperator Green's functions and a systematic procedure for treating various degrees of freedom consistently at different levels of theory is developed. The standard Fermi Golden Rule expressions for photoelectron spectra, which are limited to broad, slowly-varying signals, are obtained as a limiting case of our more general theory that applies to broader parameter regimes.

引用

页码：405 / 428

页数：24

共 53 条

[1] Resonant inelastic x-ray scattering studies of elementary excitations [J].

Ament, Luuk J. P. ;

van Veenendaal, Michel ;

Devereaux, Thomas P. ;

Hill, John P. ;

van den Brink, Jeroen .

REVIEWS OF MODERN PHYSICS, 2011, 83 (02) :705-767

[2] Newton-X: a surface-hopping program for nonadiabatic molecular dynamics [J].

Barbatti, Mario ;

Ruckenbauer, Matthias ;

Plasser, Felix ;

Pittner, Jiri ;

Granucci, Giovanni ;

Persico, Maurizio ;

Lischka, Hans .

WILEY INTERDISCIPLINARY REVIEWS-COMPUTATIONAL MOLECULAR SCIENCE, 2014, 4 (01) :26-33

[3] Time-, frequency-, and wavevector-resolved x-ray diffraction from single molecules [J].

Bennett, Kochise ;

Biggs, Jason D. ;

Zhang, Yu ;

Dorfman, Konstantin E. ;

Mukamel, Shaul .

JOURNAL OF CHEMICAL PHYSICS, 2014, 140 (20)

[4] Multidimensional scattering of attosecond x-ray pulses detected by photon-coincidence [J].

Biggs, Jason D. ;

Bennett, Kochise ;

Zhang, Yu ;

Mukamel, Shaul .

JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2014, 47 (12)

[5] Coherent nonlinear optical studies of elementary processes in biological complexes: diagrammatic techniques based on the wave function versus the density matrix [J].

Biggs, Jason D. ;

Voll, Judith A. ;

Mukamel, Shaul .

PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES, 2012, 370 (1972) :3709-3727

[6] Ultrafast X-ray absorption spectroscopy [J].

Bressler, C ;

Chergui, M .

CHEMICAL REVIEWS, 2004, 104 (04) :1781-1812

[7]

Cederbaum L. S., 1977, ADV CHEM PHYS, V36, P205, DOI DOI 10.1002/9780470142554.ch4

[8] Femtosecond diffractive imaging with a soft-X-ray free-electron laser [J].

Chapman, Henry N. ;

Barty, Anton ;

Bogan, Michael J. ;

Boutet, Sebastien ;

Frank, Matthias ;

Hau-Riege, Stefan P. ;

Marchesini, Stefano ;

Woods, Bruce W. ;

Bajt, Sasa ;

Benner, Henry ;

London, Richard A. ;

Ploenjes, Elke ;

Kuhlmann, Marion ;

Treusch, Rolf ;

Duesterer, Stefan ;

Tschentscher, Thomas ;

Schneider, Jochen R. ;

Spiller, Eberhard ;

Moeller, Thomas ;

Bostedt, Christoph ;

Hoener, Matthias ;

Shapiro, David A. ;

Hodgson, Keith O. ;

Van der Spoel, David ;

Burmeister, Florian ;

Bergh, Magnus ;

Caleman, Carl ;

Huldt, Goesta ;

Seibert, M. Marvin ;

Maia, Filipe R. N. C. ;

Lee, Richard W. ;

Szoeke, Abraham ;

Timneanu, Nicusor ;

Hajdu, Janos .

NATURE PHYSICS, 2006, 2 (12) :839-843

[9] Femtosecond X-ray protein nanocrystallography [J].

Chapman, Henry N. ;

Fromme, Petra ;

Barty, Anton ;

White, Thomas A. ;

Kirian, Richard A. ;

Aquila, Andrew ;

Hunter, Mark S. ;

Schulz, Joachim ;

DePonte, Daniel P. ;

Weierstall, Uwe ;

Doak, R. Bruce ;

Maia, Filipe R. N. C. ;

Martin, Andrew V. ;

Schlichting, Ilme ;

Lomb, Lukas ;

Coppola, Nicola ;

Shoeman, Robert L. ;

Epp, Sascha W. ;

Hartmann, Robert ;

Rolles, Daniel ;

Rudenko, Artem ;

Foucar, Lutz ;

Kimmel, Nils ;

Weidenspointner, Georg ;

Holl, Peter ;

Liang, Mengning ;

Barthelmess, Miriam ;

Caleman, Carl ;

Boutet, Sebastien ;

Bogan, Michael J. ;

Krzywinski, Jacek ;

Bostedt, Christoph ;

Bajt, Sasa ;

Gumprecht, Lars ;

Rudek, Benedikt ;

Erk, Benjamin ;

Schmidt, Carlo ;

Hoemke, Andre ;

Reich, Christian ;

Pietschner, Daniel ;

Strueder, Lothar ;

Hauser, Guenter ;

Gorke, Hubert ;

Ullrich, Joachim ;

Herrmann, Sven ;

Schaller, Gerhard ;

Schopper, Florian ;

Soltau, Heike ;

Kuehnel, Kai-Uwe ;

Messerschmidt, Marc .

NATURE, 2011, 470 (7332) :73-U81

[10] X-ray imaging beyond the limits [J].

Chapman, Henry N. .

NATURE MATERIALS, 2009, 8 (04) :299-301

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