Meteorological factors contributing to organic and elemental carbon concentrations in PM10 near an open-pit coal mine

被引:7
作者
Arregoces, Heli A. [1 ,2 ]
Rojano, Roberto [1 ]
Restrepo, Gloria [2 ]
机构
[1] Univ La Guajira, Fac Ingn, Grp Invest GISA, Riohacha, Colombia
[2] Univ Antioquia SIU UdeA, Fac Ingn, Grp Proc Fisicoquim Aplicados, Calle 70 52-21, Medellin, Colombia
关键词
Biomass burning; Carbonaceous aerosols; Coal; Elemental carbon; Open-pit mining; Organic carbon; FINE PARTICULATE MATTER; SOURCE APPORTIONMENT; BLACK CARBON; CHEMICAL-COMPOSITION; SEASONAL-VARIATIONS; AIRBORNE PARTICLES; SOURCE PROFILES; PM2.5; AEROSOLS; EMISSIONS;
D O I
10.1007/s11356-022-18505-7
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Variations in the carbonaceous aerosol contents, organic carbon (OC) and elemental carbon (EC), in particulate matter less than 10 mu m in size (PM10), were analyzed at sites influenced by coal mining in an open-pit mine located in northern Colombia. Samples were collected during different seasonal periods throughout 2015. Meteorological variables for each site were examined during the different seasons. Aerosols were detected using a thermal-optical reflectance protocol method. The highest PM10 concentrations, between the ranges of 28.2 +/- 8.2 mu g m(-3) and 75.0 +/- 36.5 mu g m(-3), were recorded during the dry season. However, the highest concentrations of OC (4.8-14.2 mu g m(-3)) and EC (2.9-13.9 mu g m(-3)) in PM10 were observed during the transition period between the dry and wet seasons. The strong correlation between OC and EC in PM10 (r = 0.6-1.0) during the transition season indicates a common primary combustion source. High OC (> 8.3 mu g m(-3)) and EC (> 6.9 mu g m(-3)) concentrations were associated with low wind speeds (< 2.1 m s(-1)) moving in different directions. Analyses of the sources of atmospheric aerosol pollutants in the mining area in northern Colombia showed that the daily maximum total carbon concentrations were mainly associated with regional atmospheric transport of particulate matter from industrial areas and biomass burning sites located in the territory of Venezuela.
引用
收藏
页码:28854 / 28865
页数:12
相关论文
共 68 条
  • [1] Elemental carbon deposition to Svalbard snow from Norwegian settlements and long-range transport
    Aamaas, Borgar
    Boggild, Carl Egede
    Stordal, Frode
    Berntsen, Terje
    Holmen, Kim
    Strom, Johan
    [J]. TELLUS SERIES B-CHEMICAL AND PHYSICAL METEOROLOGY, 2011, 63 (03): : 340 - 351
  • [2] A systematic review on global pollution status of particulate matter-associated potential toxic elements and health perspectives in urban environment
    Ali, Muhammad Ubaid
    Liu, Guijian
    Yousaf, Balal
    Ullah, Habib
    Abbas, Qumber
    Munir, Mehr Ahmad Mujtaba
    [J]. ENVIRONMENTAL GEOCHEMISTRY AND HEALTH, 2019, 41 (03) : 1131 - 1162
  • [3] The Unintended Impact of Colombia's Covid-19 Lockdown on Forest Fires
    Amador-Jimenez, Monica
    Millner, Naomi
    Palmer, Charles
    Pennington, R. Toby
    Sileci, Lorenzo
    [J]. ENVIRONMENTAL & RESOURCE ECONOMICS, 2020, 76 (04) : 1081 - 1105
  • [4] Atmospheric aerosols: Biogeochemical sources and role in atmospheric chemistry
    Andreae, MO
    Crutzen, PJ
    [J]. SCIENCE, 1997, 276 (5315) : 1052 - 1058
  • [5] [Anonymous], 1995, Compilation of Air Pollutant Emission factors, VI
  • [6] ARAL MM, 2010, ENV MOD HLTH RISK, P1
  • [7] Changing patterns of fire occurrence in proximity to forest edges, roads and rivers between NW Amazonian countries
    Armenteras, Dolors
    Sebastian Barreto, Joan
    Tabor, Karyn
    Molowny-Horas, Roberto
    Retana, Javier
    [J]. BIOGEOSCIENCES, 2017, 14 (11) : 2755 - 2765
  • [8] Atmospheric Particulate Pollutants and their Relationship with Meteorology in Ahmedabad
    Bhaskar, B. Vijay
    Mehta, Vikram M.
    [J]. AEROSOL AND AIR QUALITY RESEARCH, 2010, 10 (04) : 301 - 315
  • [9] Characteristics of Carbonaceous Matter in Aerosol from Selected Urban and Rural Areas of Southern Poland
    Blaszczak, Barbara
    Mathews, Barbara
    [J]. ATMOSPHERE, 2020, 11 (07)
  • [10] Ambient site, home outdoor and home indoor particulate concentrations as proxies of personal exposures
    Brown, Kathleen Ward
    Sarnat, Jeremy A.
    Suh, Helen H.
    Coull, Brent A.
    Spengler, John D.
    Koutrakis, Petros
    [J]. JOURNAL OF ENVIRONMENTAL MONITORING, 2008, 10 (09): : 1041 - 1051