Theoretical study of above-threshold dissociation on diatomic molecules by using nonresonant intense laser pulses

被引：12

作者：

Sugimori, Kimikazu ^{[1
]}

Ito, Tomoya

Takata, Yusuke

Ichitani, Kazuhiro

Nagao, Hiderni

Nishikawa, Kiyoshi

机构：

[1] Kinjo Univ, Haku San 9248511, Japan

[2] Kanazawa Univ, Grad Sch Nat Sci & Technol, Div Math & Phys Sci, Kanazawa, Ishikawa 9201192, Japan

来源：

JOURNAL OF PHYSICAL CHEMISTRY A | 2007年 / 111卷 / 38期

关键词：

D O I：

10.1021/jp074071x

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The above-threshold dissociation of the ground state of a OH molecule under intense nonresonant laser pulses has been studied using the time-dependent Schrodinger equation with discrete variable representation. The applied field is assumed as a two-color mixed nonresonant laser pulses which has the nonresonant frequency omega and the overtone 2 omega. After modulating the relative phase factor between the omega and 2 omega pulse, we extracted a three-photon absorption peak or a five-photon absorption peak in the ATD spectrum.

引用

页码：9417 / 9423

页数：7

共 41 条

[1] Coherent population transfer among quantum states of atoms and molecules
Bergmann, K
Theuer, H
Shore, BW
[J]. REVIEWS OF MODERN PHYSICS, 1998, 70 (03) : 1003 - 1025
[2] BISSELING RH, 1985, J CHEM PHYS, V83, P993, DOI 10.1063/1.449426
[3] SOFTENING OF THE H2+ MOLECULAR-BOND IN INTENSE LASER FIELDS
BUCKSBAUM, PH
ZAVRIYEV, A
MULLER, HG
SCHUMACHER, DW
[J]. PHYSICAL REVIEW LETTERS, 1990, 64 (16) : 1883 - 1886
[4] COHERENT POPULATION TRANSFER VIA THE CONTINUUM
CARROLL, CE
HIOE, FT
[J]. PHYSICAL REVIEW LETTERS, 1992, 68 (24) : 3523 - 3526
[5] Transferring vibrational population between electronic states of diatomic molecules via light-induced-potential shaping
Chang, BY
Solá, IR
Santamaría, J
Malinovsky, VS
Krause, JL
[J]. JOURNAL OF CHEMICAL PHYSICS, 2001, 114 (20) : 8820 - 8830
[6] ADIABATIC CLIMBING OF VIBRATIONAL LADDERS USING RAMAN TRANSITIONS WITH A CHIRPED PUMP LASER
CHELKOWSKI, S
GIBSON, GN
[J]. PHYSICAL REVIEW A, 1995, 52 (05): : R3417 - R3420
[7] NOISE-FREE SPECTRUM FOR TIME-DEPENDENT CALCULATION OF EIGENENERGIES
DAI, JQ
ZHANG, JZH
[J]. JOURNAL OF CHEMICAL PHYSICS, 1995, 103 (04) : 1491 - 1497
[8] FEIT MD, 1983, J CHEM PHYS, V78, P301, DOI 10.1063/1.444501
[9] SOLUTION OF THE SCHRODINGER-EQUATION BY A SPECTRAL METHOD
FEIT, MD
FLECK, JA
STEIGER, A
[J]. JOURNAL OF COMPUTATIONAL PHYSICS, 1982, 47 (03) : 412 - 433
[10] FRISCH MJ, 2004, GAUSSIAN 03 REVISIOJ

← 1 2 3 4 5 →