Transparent Perovskite Light-Emitting Touch-Responsive Device

被引:43
作者
Chou, Shu-Yu [1 ]
Ma, Rujun [1 ]
Li, Yunfei [1 ,2 ]
Zhao, Fangchao [1 ]
Tong, Kwing [1 ]
Yu, Zhibin [3 ]
Pei, Qibing [1 ]
机构
[1] Univ Calif Los Angeles, Dept Mat Sci & Engn, Henry Samueli Sch Engn & Appl Sci, Los Angeles, CA 90095 USA
[2] Jilin Univ, Dept Elect Sci & Engn, State Key Lab Integrated Optoelect, Changchun 130012, Jilin, Peoples R China
[3] Florida State Univ, Dept Ind & Mfg Engn, High Performance Mat Inst, FAMU FSU Coll Engn, Tallahassee, FL 32310 USA
关键词
touch response; light emitting; perovskite; flexible; transparent; silver nanowires; HALIDE PEROVSKITE; SOLAR-CELLS; IMPROVED PERFORMANCE; HIGH-EFFICIENCY; DIODES; ELECTRODES; LAYER; FILMS; BRIGHTNESS; TACTILE;
D O I
10.1021/acsnano.7b05935
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A light-emitting touch-responsive device (LETD) for instantaneous visualization of pressure mapping is reported. The LETD integrates an organometal halide perovskite polymer composite emissive layer and a flexible silver nanowire polyurethane composite transparent electrode. The composite emissive layer contains methyl ammonium lead bromide nanocrystals uniformly dispersed in a poly(ethylene oxide) (PEO) matrix and emits an intense green luminescence that peaks at 529 nm. The PEO matrix promotes the formation of small perovskite grains (similar to 20 nm) and a pinhole-free composite film with surface roughness of only 2.96 nm. The composite transparent electrode is separated from the emissive layer with a 100 mu m thick spacer. When a local pressure is applied, a Schottky contact is formed instantaneously between the metal and the emissive layer, and electroluminescence is produced at voltages as low as 2.5 V and reaches 1030 cd/m(2) at 6 V. The transparent LETD has approximately 68% transparency. It can be bent to a 6 mm radius when polyethylene terephthalate is used as the substrate. The perovskite LETD has fast response and can be pixelated to offer potential applications in robotics, motion detection, fingerprint devices, and interactive wallpapers.
引用
收藏
页码:11368 / 11375
页数:8
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