Enhancing High Harmonic Output in Solids through Quantum Confinement

被引:45
作者
McDonald, C. R. [1 ]
Amin, K. S. [1 ]
Aalmalki, S. [1 ]
Brabec, T. [1 ]
机构
[1] Univ Ottawa, Dept Phys, Ottawa, ON K1N 6N5, Canada
关键词
DYNAMICS; FIELD; GENERATION; ENERGY;
D O I
10.1103/PhysRevLett.119.183902
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We investigate theoretically the effect of quantum confinement on high harmonic generation (HHG) in semiconductors by systematically varying the width of a model quantum nanowire. Our analysis reveals a reduction in ionization and a concurrent growth in HHG efficiency with increasing confinement. The drop in ionization results from an increase in the band gap due to stronger confinement. The increase in harmonic efficiency comes as a result of the confinement restricting the spreading of the transverse wave packet. As a result, intense laser driven 1D and 2D nanosystems present a potential pathway to increasing yield and photon energy of HHG in solids.
引用
收藏
页数:6
相关论文
共 36 条
[1]   Probing proton dynamics in molecules on an attosecond time scale [J].
Baker, S ;
Robinson, JS ;
Haworth, CA ;
Teng, H ;
Smith, RA ;
Chirila, CC ;
Lein, M ;
Tisch, JWG ;
Marangos, JP .
SCIENCE, 2006, 312 (5772) :424-427
[2]   Exciton Binding Energy and Nonhydrogenic Rydberg Series in Monolayer WS2 [J].
Chernikov, Alexey ;
Berkelbach, Timothy C. ;
Hill, Heather M. ;
Rigosi, Albert ;
Li, Yilei ;
Aslan, Ozgur Burak ;
Reichman, David R. ;
Hybertsen, Mark S. ;
Heinz, Tony F. .
PHYSICAL REVIEW LETTERS, 2014, 113 (07)
[3]   Attosecond science [J].
Corkum, P. B. ;
Krausz, Ferenc .
NATURE PHYSICS, 2007, 3 (06) :381-387
[4]   PLASMA PERSPECTIVE ON STRONG-FIELD MULTIPHOTON IONIZATION [J].
CORKUM, PB .
PHYSICAL REVIEW LETTERS, 1993, 71 (13) :1994-1997
[5]   Gauge invariance and interpretation of interband and intraband processes in high-order harmonic generation from bulk solids [J].
Foeldi, Peter .
PHYSICAL REVIEW B, 2017, 96 (03)
[6]   Observation of high-order harmonic generation in a bulk crystal [J].
Ghimire, Shambhu ;
DiChiara, Anthony D. ;
Sistrunk, Emily ;
Agostini, Pierre ;
DiMauro, Louis F. ;
Reis, David A. .
NATURE PHYSICS, 2011, 7 (02) :138-141
[7]   High harmonics generated in semiconductor nanostructures by the coupled dynamics of optical inter- and intraband excitations [J].
Golde, D. ;
Meier, T. ;
Koch, S. W. .
PHYSICAL REVIEW B, 2008, 77 (07)
[8]   Role of subcycle transition dynamics in high-order-harmonic generation in periodic structures [J].
Hawkins, Peter G. ;
Ivanov, Misha Yu .
PHYSICAL REVIEW A, 2013, 87 (06)
[9]   Tightly Bound Excitons in Monolayer WSe2 [J].
He, Keliang ;
Kumar, Nardeep ;
Zhao, Liang ;
Wang, Zefang ;
Mak, Kin Fai ;
Zhao, Hui ;
Shan, Jie .
PHYSICAL REVIEW LETTERS, 2014, 113 (02)
[10]  
Higuchi T., ARXIV160704198V1