Electron dipole-dipole interaction in ESEEM of nitroxide biradicals

被引：168

作者：

Kulik, LV

Dzuba, SA

Grigoryev, IA

Tsvetkov, YD

机构：

[1] Russian Acad Sci, Inst Chem Kinet & Combust, Novosibirsk 630090, Russia

[2] Novosibirsk State Univ, Novosibirsk 630090, Russia

[3] Russian Acad Sci, Novosibirsk Organ Chem Inst, Novosibirsk 630090, Russia

来源：

CHEMICAL PHYSICS LETTERS | 2001年 / 343卷 / 3-4期

基金：

俄罗斯基础研究基金会;

关键词：

D O I：

10.1016/S0009-2614(01)00721-7

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Fourier transform of the standard primary electron spin echo envelope modulation (ESEEM) of nitroxide biradicals in organic glass shows a peak ascribed to electron-electron dipole-dipole interaction. The dipolar couplings obtained in imidazoline biradical and double spin-labeled peptide Trichogin GA IV are in good agreement with pulsed electron-electron double resonance (PELDOR) data. The intensity of this peak is increased substantially in a new three-pulse relaxation-induced dipolar modulation enhancement (RIDME) experiment, This experiment involves the non-resonant partner spin in the formation of ESEEM via a relaxation-induced change of the local dipolar field experienced by the resonant spin. (C) 2001 Published by Elsevier Science B.V.

引用

页码：315 / 324

页数：10

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