Tailoring the Heterostructure of Colloidal Quantum Dots for Ratiometric Optical Nanothermometry

被引:45
作者
Zhao, Haiguang [1 ]
Vomiero, Alberto [2 ,3 ,4 ]
Rosei, Federico [5 ]
机构
[1] Qingdao Univ, State Key Lab Biofibers & Ecotext, 308 Ningxia Rd, Qingdao 266071, Peoples R China
[2] Qingdao Univ, Coll Phys, Univ Ind Joint Ctr Ocean Observat & Broadband Com, Qingdao 266071, Peoples R China
[3] Lulea Univ Technol, Div Mat Sci, Dept Engn Sci & Math, Lulea 97187, Sweden
[4] Ca Foscari Univ Venice, Dept Mol Sci & Nano Syst, Via Torino 155, Venice 30172, Italy
[5] Univ Quebec, Inst Natl Rech Sci, Ctr Energy Mat & Telecommun, 1650 Blvd Lionel Boulet, Varennes, PQ J3X 1S2, Canada
基金
加拿大自然科学与工程研究理事会; 欧盟地平线“2020”;
关键词
dual-emission quantum dots (QDs); heterostructures; nanothermometry; thermal sensitivity; thermal sensors; LUMINESCENT SOLAR CONCENTRATORS; DUAL-EMISSION; CARBON-DOTS; FLUORESCENT NANOTHERMOMETERS; CATION-EXCHANGE; NANOCRYSTALS; CDSE/CDS; PHOTOLUMINESCENCE; EFFICIENT; THERMOMETRY;
D O I
10.1002/smll.202000804
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Colloidal quantum dots (QDs) are a fascinating class of semiconducting nanocrystals, thanks to their optical properties tunable through size and composition, and simple synthesis methods. Recently, colloidal double-emission QDs have been successfully applied as competitive optical temperature sensors, since they exhibit structure-tunable double emission, temperature-dependent photoluminescence, high quantum yield, and excellent photostability. Until now, QDs have been used as nanothermometers for in vivo biological thermal imaging, and thermal mapping in complex environments at the sub-microscale to nanoscale range. In this Review, recent progress for QD-based nanothermometers is highlighted and perspectives for future work are described.
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页数:18
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共 128 条
[1]   Heterostructured quantum dot architectures for efficient and stable photoelectrochemical hydrogen production [J].
Adhikari, Rajesh ;
Basu, Kaustubh ;
Zhou, Yufeng ;
Vetrone, Fiorenzo ;
Ma, Dongling ;
Sun, Shuhui ;
Vidal, Francois ;
Zhao, Haiguang ;
Rosei, Federico .
JOURNAL OF MATERIALS CHEMISTRY A, 2018, 6 (16) :6822-6829
[2]   Dual-Emitting Quantum Dot/Quantum Rod-Based Nanothermometers with Enhanced Response and Sensitivity in Live Cells [J].
Albers, Aaron E. ;
Chan, Emory M. ;
McBride, Patrick M. ;
Ajo-Franklin, Caroline M. ;
Cohen, Bruce E. ;
Helms, Brett A. .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2012, 134 (23) :9565-9568
[3]   Semiconductor clusters, nanocrystals, and quantum dots [J].
Alivisatos, AP .
SCIENCE, 1996, 271 (5251) :933-937
[4]   Inorganic cluster syntheses of TM2+-doped quantum dots (CdSe, CdS, CdSe/CdS):: Physical property dependence on dopant locale [J].
Archer, Paul I. ;
Santangelo, Steven A. ;
Gamelin, Daniel R. .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (31) :9808-9818
[5]   Direct observation of sp-d exchange interactions in colloidal Mn2+- and Co2+-doped CdSe quantum dots [J].
Archer, Paul I. ;
Santangelo, Steven A. ;
Gamelin, Daniel R. .
NANO LETTERS, 2007, 7 (04) :1037-1043
[6]   Controlled Alloying of the Core-Shell Interface in CdSe/CdS Quantum Dots for Suppression of Auger Recombination [J].
Bae, Wan Ki ;
Padilha, Lazaro A. ;
Park, Young-Shin ;
McDaniel, Hunter ;
Robel, Istvan ;
Pietryga, Jeffrey M. ;
Klimov, Victor I. .
ACS NANO, 2013, 7 (04) :3411-3419
[7]   Micro/Nanoscale Thermometry for Cellular Thermal Sensing [J].
Bai, Tingting ;
Gu, Ning .
SMALL, 2016, 12 (34) :4590-4610
[8]   Coupled and decoupled dual quantum systems in one semiconductor nanocrystal [J].
Battaglia, D ;
Blackman, B ;
Peng, XG .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2005, 127 (31) :10889-10897
[9]   Exciton storage by Mn2+ in colloidal Mn2+-doped CdSe quantum dots [J].
Beaulac, Remi ;
Archer, Paul I. ;
van Rijssel, Jos ;
Meijerink, Andries ;
Gamelin, Daniel R. .
NANO LETTERS, 2008, 8 (09) :2949-2953
[10]   Spin-polarizable excitonic luminescence in colloidal Mn2+-doped CdSe quantum dots [J].
Beaulac, Remi ;
Archer, Paul I. ;
Liu, Xinyu ;
Lee, Sanghoon ;
Salley, G. Mackay ;
Dobrowolska, Margaret ;
Furdyna, Jacek K. ;
Gamelin, Daniel R. .
NANO LETTERS, 2008, 8 (04) :1197-1201