A systematic generation of reactor designs II. Non-isothermal conditions

被引:14
作者
Hillestad, M [1 ]
机构
[1] Cybernet AS, N-7038 Trondheim, Norway
关键词
optimal reactor design; reactor network synthesis; the maximum principle; optimal mixing; heat transfer; distributed feed; methanol synthesis; steam methane reforming;
D O I
10.1016/j.compchemeng.2004.11.009
中图分类号
TP39 [计算机的应用];
学科分类号
081203 ; 0835 ;
摘要
A new method is proposed for systematic generation of conceptual design of reactor networks. Here, non-isothermal conditions are considered. Optimal distribution of heat transfer area, in addition to optimal mixing and distribution of feeds are targeted. Given temperature and composition of feed streams, the objective is to find the sequence and size of ideal reactors, the distribution of extra feed streams, the heat transfer distribution along the reactor path and the total reaction time that maximizes the space-time yield of the key product component. The method can be applied to solve problems of any number of components and reactions. The method is applied to industrially important processes such as the methanol synthesis and the steam methane reforming process. Interesting results are obtained with respect to the required heat exchange area. (c) 2004 Elsevier Ltd. All rights reserved.
引用
收藏
页码:1101 / 1112
页数:12
相关论文
共 12 条
[1]   CONSTRUCTIVE TARGETING APPROACHES FOR THE SYNTHESIS OF CHEMICAL REACTOR NETWORKS [J].
BALAKRISHNA, S ;
BIEGLER, LT .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1992, 31 (01) :300-312
[2]   Toward a theory of process synthesis [J].
Feinberg, M .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2002, 41 (16) :3751-3761
[3]  
FROMENT GF, 1990, CHEM REACTOR ANAL
[4]   KINETICS OF LOW-PRESSURE METHANOL SYNTHESIS [J].
GRAAF, GH ;
STAMHUIS, EJ ;
BEENACKERS, AACM .
CHEMICAL ENGINEERING SCIENCE, 1988, 43 (12) :3185-3195
[5]   A systematic generation of reactor designs - I. Isothermal conditions [J].
Hillestad, M .
COMPUTERS & CHEMICAL ENGINEERING, 2004, 28 (12) :2717-2726
[6]   Optimal reactor structures for exothermic reversible reactions with complex kinetics [J].
Hopley, F ;
Glasser, D ;
Hildebrandt, D .
CHEMICAL ENGINEERING SCIENCE, 1996, 51 (10) :2399-2407
[7]   Heterogeneous catalytic reactor design with optimum temperature profile I: application of catalyst dilution and side-stream distribution [J].
Hwang, SW ;
Smith, R .
CHEMICAL ENGINEERING SCIENCE, 2004, 59 (20) :4229-4243
[8]  
Jackson R., 1968, Journal of Optimization Theory and Applications, V2, P240, DOI 10.1007/BF00937370
[9]  
SUPP E, 1981, HYDROCARB PROCESS, V3, P71
[10]   The water-gas-shift reaction at short contact times [J].
Wheeler, C ;
Jhalani, A ;
Klein, EJ ;
Tummala, S ;
Schmidt, LD .
JOURNAL OF CATALYSIS, 2004, 223 (01) :191-199