Investigation of Porous Metal-Based 3D-Printed Anode GDLs for Tubular High Temperature Proton Exchange Membrane Fuel Cells

被引:19
作者
Agudelo, Maria Catalina Bermudez [1 ]
Hampe, Manfred [1 ]
Reiber, Thorsten [2 ]
Abele, Eberhard [2 ]
机构
[1] Tech Univ Darmstadt, Thermal Proc Engn Grp TVT, Inst Nano & Microfluid NMF, Otto Berndt Str 2, D-64287 Darmstadt, Germany
[2] Tech Univ Darmstadt, Inst Prod Management Technol & Machine Tools PTW, Otto Berndt Str 2, D-64287 Darmstadt, Germany
关键词
additive manufacturing; gas diffusion layer (GDL); high-temperature proton exchange membrane fuel cell (HT-PEMFC); MEA preparation; porosity; powder bed fusion using a laser beam (PBF-LB); tubular design; 316L STAINLESS-STEEL; BIPOLAR PLATE MATERIAL; GAS-DIFFUSION LAYERS; MECHANICAL-PROPERTIES; CORROSION BEHAVIOR; DENSITY; DESIGN;
D O I
10.3390/ma13092096
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A high-temperature proton exchange membrane fuel cell (HT-PEMFC) conventionally uses a planar design with carbon-based substrates as the gas diffusion layer (GDL) materials. However, the metal-based substrates allow for alternative designs. In this study, the applicability of porous thin-walled tubular elements made of 316L stainless steel as the anode GDL in a multi-layer tubular HT-PEMFC was investigated. The anode GDLs were fabricated via powder bed fusion using a laser beam (PBF-LB) process with defined porosities (14% and 16%). The morphology of the porous elements was compared using scanning electron microscopy (SEM) micrographs. The influence of the porosity on the fuel cell performance was evaluated through electrochemical characterization and a short-term stability test (45 h) in a commercial test station operated at 160 degrees C and ambient pressure, using hydrogen as the fuel and air as the oxidant. The results showed that the fuel cell manufactured upon the anode GDL with a porosity of 16% had a higher performance with a peak power density of 329.25 W/m(2) after 5 h of operation at 125.52 A/m(2) and a voltage degradation rate of 0.511 mV/h over the stability test period. Moreover, this work indicates that additive manufacturing could be a useful tool for further fuel cell development.
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页数:12
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