Wafer-Scale InN/In2S3 Core-Shell Nanorod Array for Ultrafast Self-Powered Photodetection

被引:23
作者
Cao, Ben [1 ,2 ]
Liu, Qianhu [1 ]
Zheng, Yulin [1 ]
Tang, Xin [1 ]
Chai, Jixing [1 ]
Ma, Shufang [2 ]
Wang, Wenliang [3 ]
Li, Guoqiang [3 ]
机构
[1] South China Univ Technol, Sch Mat Sci & Engn, State Key Lab Luminescent Mat & Devices, Guangzhou 510640, Peoples R China
[2] Shaanxi Univ Sci & Technol, Inst Atom & Mol Sci, Xian 710021, Peoples R China
[3] South China Univ Technol, Sch Mat Sci & Engn, Dept Elect Mat, State Key Lab Luminescent Mat & Devices, Guangzhou 510640, Peoples R China
基金
中国国家自然科学基金;
关键词
core-shell nanorods; InN; In; S-2; (3); self-powered photodetectors; ultrafast photodetection; wafer-scale; INN; GROWTH; GAS;
D O I
10.1002/adfm.202110715
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Self-powered photodetectors have paved the way for electronic applications in fields such as civilian communication, infrared mapping, and industrial automatic control. However, most self-powered photodetectors have faced photoresponse-speed and device-scale bottlenecks. Herein, a novel, self-powered detector with an ultrafast response speed based on a core-shell InN/In2S3 nanorod array is proposed. A wafer-scale InN/In2S3 nanorod array with good homogeneity is synthesized on Si substrates via a simple two-step method involving molecular beam epitaxy and chemical vapor deposition. The photodetector device exhibits excellent self-powered properties and a high current on/off ratio of 5 x 10(3). Further analyses determined that the device have an excellent photovoltaic responsivity and detectivity of 140 mA center dot W-1 and 4.0 x 10(10) Jones, respectively (0 V). Impressively, the device exhibits an ultrafast photoresponse with a rise/fall time of 22/32 mu s. The self-powered InN/In2S3 photodetector with an ultrafast response speed shows superior potential for electronic applications. The core-shell nanostructure hybrid heterojunction introduces a novel idea for wafer-scale nano-photodetectors.
引用
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页数:9
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