Preparation of graphene-MoS2 hybrid aerogels as multifunctional sorbents for water remediation

被引:32
作者
Chen, Bo [1 ,2 ,3 ]
Bi, Hengchang [3 ,4 ]
Ma, Qinglang [1 ,2 ,3 ]
Tan, Chaoliang [3 ]
Cheng, Hongfei [3 ]
Chen, Ye [3 ]
He, Xinyan [3 ]
Sun, Litao [4 ]
Lim, Teik-Thye [1 ,5 ]
Huang, Ling [6 ,7 ]
Zhang, Hua [3 ]
机构
[1] Nanyang Technol Univ, NEWRI, Singapore 637141, Singapore
[2] Nanyang Technol Univ, IGS, Singapore 639798, Singapore
[3] Nanyang Technol Univ, Sch Mat Sci & Engn, Ctr Programmable Mat, Singapore 639798, Singapore
[4] Southeast Univ, SEU FEI Nanopico Ctr, Key Lab MEMS, Minist Educ,Collaborat Innovat Ctr Micro Nano Fab, Nanjing 210096, Jiangsu, Peoples R China
[5] Nanyang Technol Univ, Sch Civil & Environm Engn, Singapore 639798, Singapore
[6] Nanjing Tech Univ NanjingTech, KLOFE, Natl Jiangsu Synergist Innovat Ctr Adv Mat SICAM, Nanjing 211816, Peoples R China
[7] Nanjing Tech Univ NanjingTech, IAM, Natl Jiangsu Synergist Innovat Ctr Adv Mat SICAM, Nanjing 211816, Peoples R China
基金
新加坡国家研究基金会;
关键词
Graphene; MoS2; aerogels; multifunctional sorbents; water remediation; ORGANIC-SOLVENTS; RECYCLABLE SORBENT; CARBON AEROGELS; SPONGY GRAPHENE; ADSORPTION; REMOVAL; OXIDE; MOS2; EFFICIENT; SEPARATION;
D O I
10.1007/s40843-017-9150-7
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The increasing demand of clean water and effective way to recycle industrial wastewater has offered a new application for carbon-based three-dimensional (3D) porous networks as sorbents due to their superior sorption abilities. Through the surface modification and hybridization with functional materials, the physical and chemical properties of the 3D carbon-based materials can be engineered. In this work, graphene-MoS2 aerogels (GMAs) with bulky shape are synthesized via a one-pot hydrothermal method. The obtained GMAs show quick sorption rate and high sorption capacity towards a wide variety of contaminants. The sorption covers not only organic solvents or organic dyes, but also toxic heavy metals ions such as Hg2+ and Pb2+. More importantly, the sorption capacity towards metal ions can be optimized by simply changing the loading amount of MoS2.
引用
收藏
页码:1102 / 1108
页数:7
相关论文
共 33 条
[1]   MoS2 Nanosheets with Widened Interlayer Spacing for High-Efficiency Removal of Mercury in Aquatic Systems [J].
Ai, Kelong ;
Ruan, Changping ;
Shen, Mengxia ;
Lu, Lehui .
ADVANCED FUNCTIONAL MATERIALS, 2016, 26 (30) :5542-5549
[2]  
Bi HC, 2014, J MATER CHEM A, V2, P1652, DOI [10.1039/c3ta14112, 10.1039/c3ta14112h]
[3]   Carbon Fiber Aerogel Made from Raw Cotton: A Novel, Efficient and Recyclable Sorbent for Oils and Organic Solvents [J].
Bi, Hengchang ;
Yin, Zongyou ;
Cao, Xiehong ;
Xie, Xiao ;
Tan, Chaoliang ;
Huang, Xiao ;
Chen, Bo ;
Chen, Fangtao ;
Yang, Qingling ;
Bu, Xinyang ;
Lu, Xuehong ;
Sun, Litao ;
Zhang, Hua .
ADVANCED MATERIALS, 2013, 25 (41) :5916-5921
[4]   Spongy Graphene as a Highly Efficient and Recyclable Sorbent for Oils and Organic Solvents [J].
Bi, Hengchang ;
Xie, Xiao ;
Yin, Kuibo ;
Zhou, Yilong ;
Wan, Shu ;
He, Longbing ;
Xu, Feng ;
Banhart, Florian ;
Sun, Litao ;
Ruoff, Rodney S. .
ADVANCED FUNCTIONAL MATERIALS, 2012, 22 (21) :4421-4425
[5]   Application of graphene-like layered molybdenum disulfide and its excellent adsorption behavior for doxycycline antibiotic [J].
Chao, Yanhong ;
Zhu, Wenshuai ;
Wu, Xiangyang ;
Hou, Fangfang ;
Xun, Suhang ;
Wu, Peiwen ;
Ji, Haiyan ;
Xu, Hui ;
Li, Huaming .
CHEMICAL ENGINEERING JOURNAL, 2014, 243 :60-67
[6]   Carbon-Based Sorbents with Three-Dimensional Architectures for Water Remediation [J].
Chen, Bo ;
Ma, Qinglang ;
Tan, Chaoliang ;
Lim, Teik-Thye ;
Huang, Ling ;
Zhang, Hua .
SMALL, 2015, 11 (27) :3319-3336
[7]   Versatile Fabrication of Ultralight Magnetic Foams and Application for Oil-Water Separation [J].
Chen, Ning ;
Pan, Qinmin .
ACS NANO, 2013, 7 (08) :6875-6883
[8]   2D nanostructures for water purification: graphene and beyond [J].
Dervin, Saoirse ;
Dionysiou, Dionysios D. ;
Pillai, Suresh C. .
NANOSCALE, 2016, 8 (33) :15115-15131
[9]   Superhydrophobic and superoleophilic hybrid foam of graphene and carbon nanotube for selective removal of oils or organic solvents from the surface of water [J].
Dong, Xiaochen ;
Chen, Jun ;
Ma, Yanwen ;
Wang, Jing ;
Chan-Park, Mary B. ;
Liu, Xiangmei ;
Wang, Lianhui ;
Huang, Wei ;
Chen, Peng .
CHEMICAL COMMUNICATIONS, 2012, 48 (86) :10660-10662
[10]   Superhydrophobic and superoleophilic properties of graphene-based sponges fabricated using a facile dip coating method [J].
Duc Dung Nguyen ;
Tai, Nyan-Hwa ;
Lee, San-Boh ;
Kuo, Wen-Shyong .
ENERGY & ENVIRONMENTAL SCIENCE, 2012, 5 (07) :7908-7912