Numerical investigation of the impact of washcoat distribution on the filtration performance of gasoline particulate filters

被引:28
作者
Belot, Igor [1 ]
Vidal, David [1 ,2 ]
Votsmeier, Martin [3 ,4 ]
Hayes, Robert E. [5 ]
Bertrand, Francois [1 ]
机构
[1] Polytech Montreal, Res Ctr Ind Flow Proc URPEI, Dept Chem Engn, Montreal, PQ H3C 3A7, Canada
[2] Polytech Montreal, Dept Mech Engn, Montreal, PQ H3C 3A7, Canada
[3] UMICORE AG & Co KG, Rodenbacher Chausee 4, D-63457 Hanau, Germany
[4] Tech Univ Darmstadt, Ernst Berl Inst Tech & Makromol Chem, Alarich Weiss Str 8, D-64287 Darmstadt, Germany
[5] Univ Alberta, Dept Mech Engn, Edmonton, AB T6G 2G6, Canada
基金
加拿大自然科学与工程研究理事会;
关键词
Gasoline particulate filter; Three-way catalyst uniformity; Soot filtration; Structure reconstruction; Porous media; Lattice Boltzmann method; SELECTIVE CATALYTIC-REDUCTION; PRESSURE-DROP; SIMULATION; PERMEABILITY; REGENERATION; TECHNOLOGY; EFFICIENCY; PARTICLES; EMISSIONS; MEDIA;
D O I
10.1016/j.ces.2020.115656
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
A three-step numerical model sheds light on the impact of three-way catalyst washcoat distribution within the cordierite porous wall of a clean gasoline particulate filter on its filtration performance. The model relies on (1) the numerical reconstruction of porous wall sections with various washcoat distributions and coating amounts, generated using a novel set of morphological image processing operations applied on segmented X-ray computed tomography data, (2) the computation of the flow field using the lattice Boltzmann method, and (3) the prediction of soot capture efficiency by solving the Langevin equation. The impact of washcoat distribution and amount on the pressure drop, permeability, filtration efficiency, and filter quality factor is systematically investigated. For a non-uniform washcoat distribution, an unexpected decrease in filtration efficiency with an increase in washcoat amount is explained and this highlights the complexity of the effects generated by the deposition of washcoat within the porous wall of the filter. (C) 2020 Elsevier Ltd. All rights reserved.
引用
收藏
页数:19
相关论文
共 83 条
[1]  
Aderhold Dirk., 1999, International Search Report
[2]  
[Anonymous], 2006, TRANSPORT PHENOMENA
[3]  
Azimian M., 2017, CHALL EXH AFR DIES E
[4]   Simulation of Cake Filtration for Polydisperse Particles [J].
Becker, Juergen ;
Cheng, Liping ;
Kronsbein, Cornelia ;
Wiegmann, Andreas .
CHEMICAL ENGINEERING & TECHNOLOGY, 2016, 39 (03) :559-566
[5]  
Belot I., 2020, CHEM ENG SC
[6]  
Belot Igor., 2020, Chemical Engineering Journal
[7]   Modelling of diesel particulate filtration in wall-flow traps [J].
Bensaid, S. ;
Marchisio, D. L. ;
Fino, D. ;
Saracco, G. ;
Specchia, V. .
CHEMICAL ENGINEERING JOURNAL, 2009, 154 (1-3) :211-218
[8]   Towards the simulation of the catalytic monolith converter using discrete channel-scale models [J].
Bertrand, Francois ;
Devals, Christophe ;
Vidal, David ;
de Preval, Cyrille Seguineau ;
Hayes, Robert E. .
CATALYSIS TODAY, 2012, 188 (01) :80-86
[9]   THERMAL REGENERATION OF DIESEL-PARTICULATE MONOLITHIC FILTERS [J].
BISSETT, EJ ;
SHADMAN, F .
AICHE JOURNAL, 1985, 31 (05) :753-758
[10]  
Blake FC, 1921, T AM INST CHEM ENG, V14, P415