High-precision osmium isotopes in enstatite and Rumuruti chondrites

被引:36
作者
van Acken, David [1 ,2 ]
Brandon, Alan D. [1 ]
Humayun, Munir [3 ,4 ]
机构
[1] Univ Houston, Dept Earth & Atmospher Sci, Houston, TX 77204 USA
[2] NASA, Lyndon B Johnson Space Ctr, MS KR, Houston, TX 77058 USA
[3] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA
[4] Florida State Univ, Dept Earth Ocean & Atmospher Sci, Tallahassee, FL 32310 USA
关键词
EARLY SOLAR-SYSTEM; SILICON-CARBIDE GRAINS; PLATINUM-GROUP ELEMENTS; R-PROCESS COMPONENTS; GIANT BRANCH STARS; S-PROCESS; CARBONACEOUS CHONDRITES; PRIMITIVE CHONDRITES; MURCHISON METEORITE; NEUTRON-CAPTURE;
D O I
10.1016/j.gca.2011.04.019
中图分类号
P3 [地球物理学]; P59 [地球化学];
学科分类号
0708 ; 070902 ;
摘要
Isotopic heterogeneity within the solar nebula has been a long-standing issue. Studies on primitive chondrites and chondrite components for Ba, Sm, Nd, Mo, Ru, Hf, Ti, and Os yielded conflicting results, with some studies suggesting large-scale heterogeneity. Low-grade enstatite and Rumuruti chondrites represent the most extreme ends of the chondrite meteorites in terms of oxidation state, and might thus also present extremes if there is significant isotopic heterogeneity across the region of chondrite formation. Osmium is an ideal tracer because of its multiple isotopes generated by a combination of p-, r-, and s-process and, as a refractory element; it records the earliest stages of condensation. Some grade 3-4 enstatite and Rumuruti chondrites show similar deficits of s-process components as revealed by high-precision Os isotope studies in some low-grade carbonaceous and ordinary chondrites. Enstatite chondrites of grades 5-6 have Os isotopic composition identical within error to terrestrial and solar composition. This supports the view of digestion-resistant presolar grains, most likely SiC, as the major carrier of these anomalies. Destruction of presolar grains during parent body processing, which all high-grade enstatite chondrites, but also some low-grade chondrites seemingly underwent, makes the isotopically anomalous Os accessible for analysis. The magnitude of the anomalies is consistent with the presence of a few ppm of presolar SiC with a highly unusual isotopic composition, produced in a different stellar environment like asymptotic giant branch stars (AGB) and injected into the solar nebula. The presence of similar Os isotopic anomalies throughout all major chondrite groups implies that carriers of Os isotopic anomalies were homogeneously distributed in the solar nebula, at least across the formation region of chondrites. (C) 2011 Elsevier Ltd. All rights reserved.
引用
收藏
页码:4020 / 4036
页数:17
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