Selection of organic process and source indicator substances for the anthropogenically influenced water cycle

被引:132
作者
Jekel, Martin [1 ]
Dott, Wolfgang [2 ]
Bergmann, Axel [3 ]
Duennbier, Uwe [4 ]
Gnirss, Regina [4 ]
Haist-Gulde, Brigitte [5 ]
Hamscher, Gerd [6 ]
Letzel, Marion [7 ]
Licha, Tobias [8 ]
Lyko, Sven [9 ]
Miehe, Ulf [10 ]
Sacher, Frank [5 ]
Scheurer, Marco [5 ]
Schmidt, Carsten K. [11 ]
Reemtsma, Thorsten [12 ]
Ruhl, Aki Sebastian [1 ]
机构
[1] Tech Univ Berlin, Ctr Water Urban Areas, Sekr KF4,Str 17, D-10623 Berlin, Germany
[2] Rhein Westfal TH Aachen, Inst Hyg & Environm Med, D-52074 Aachen, Germany
[3] IWW Water Ctr, Water Resources Management, D-45476 Mulheim An Der Ruhr, Germany
[4] Berliner Wasserbetriebe, D-10179 Berlin, Germany
[5] Technol Zentrum Wasser TZW, DVGW, D-76139 Karlsruhe, Germany
[6] Univ Giessen, Inst Food Chem & Food Biotechnol, D-35392 Giessen, Germany
[7] Bavarian Environm Agcy, D-82407 Wielenbach, Germany
[8] Univ Gottingen, Dept Appl Geol, Geosci Ctr, D-37077 Gottingen, Germany
[9] Emschergenossenschaft, D-45128 Essen, Germany
[10] Berlin Ctr Competence Water, D-10709 Berlin, Germany
[11] RheinEnergie AG, D-50823 Cologne, Germany
[12] UFZ Helmholtz Ctr Environm Res, Dept Analyt Chem, D-04318 Leipzig, Germany
关键词
Urban water cycle; Trace pollutants; Pharmaceuticals; Aquatic environment; Diclofenac; Sulfamethoxazole; PERSONAL CARE PRODUCTS; MUNICIPAL WASTE-WATER; PERFORMANCE LIQUID-CHROMATOGRAPHY; ENDOCRINE DISRUPTING COMPOUND; POWDERED ACTIVATED CARBON; BETA-LACTAM ANTIBIOTICS; TREATMENT PLANTS; ARTIFICIAL SWEETENERS; DRINKING-WATER; AQUATIC ENVIRONMENT;
D O I
10.1016/j.chemosphere.2014.12.025
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
An increasing number of organic micropollutants (OMP) is detected in anthropogenically influenced water cycles. Source control and effective natural and technical barriers are essential to maintain a high quality of drinking water resources under these circumstances. Based on the literature and our own research this study proposes a limited number of OMP that can serve as indicator substances for the major sources of OMP, such as wastewater treatment plants, agriculture and surface runoff. Furthermore functional indicators are proposed that allow assessment of the proper function of natural and technical barriers in the aquatic environment, namely conventional municipal wastewater treatment, advanced treatment (ozonation, activated carbon), bank filtration and soil aquifer treatment as well as self-purification in surface water. These indicator substances include the artificial sweetener acesulfame, the anti-inflammatory drug ibuprofen, the anticonvulsant carbamazepine, the corrosion inhibitor benzotriazole and the herbicide mecoprop among others. The chemical indicator substances are intended to support comparisons between watersheds and technical and natural processes independent of specific water cycles and to reduce efforts and costs of chemical analyses without losing essential information. (C) 2014 Elsevier Ltd. All rights reserved.
引用
收藏
页码:155 / 167
页数:13
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