High-efficiency removal of lead/cadmium from wastewater by MgO modified biochar derived from crofton weed

被引:138
作者
Cheng, Song [1 ,3 ]
Zhao, Saidan [1 ]
Guo, Hui [2 ,3 ]
Xing, Baolin [1 ,3 ]
Liu, Yongzhi [1 ]
Zhang, Chuanxiang [1 ,3 ]
Ma, Mingjie [1 ]
机构
[1] Henan Polytech Univ, Coll Chem & Chem Engn, Henan Key Lab Coal Green Convers, Jiaozuo 454003, Henan, Peoples R China
[2] Henan Polytech Univ, Sch Mat Sci & Engn, Jiaozuo 454003, Henan, Peoples R China
[3] Collaborat Innovat Ctr Coal Work Safety & Clean H, Jiaozuo 454003, Henan, Peoples R China
基金
中国国家自然科学基金;
关键词
Crofton weed; Pb2+/Cd2+; Adsorption; Mechanism; Column experiment; COMPETITIVE ADSORPTION; SORPTION MECHANISMS; AQUEOUS-SOLUTION; HEAVY-METALS; PB(II); CU(II); CD(II);
D O I
10.1016/j.biortech.2021.126081
中图分类号
S2 [农业工程];
学科分类号
0828 ;
摘要
The adsorption performance and mechanisms of Pb2+ and Cd2+ in wastewater using MgO modified biochar derived from crofton weed (MBCW600) are investigated. The Pb2+ and Cd2+ adsorption capacities of MBCW600 by the Hill model reach 384.08 mg/g and 207.02 mg/g, respectively, which is larger than that of original biochar. Pb2+ could be more easily captured by MBCW600 compared to Cd2+ in the multimetal system. Mg2+ contributes to Pb2+ and Cd2+ adsorption among coexisting cations. The exhausted MBCW600 could be well regenerated by simple method after use. The adsorption mechanism study indicates that Pb2+ and Cd2+ removal are primary contributed to mineral precipitation and ion exchange. The effective treatment volumes of Pb2+ and Cd2+ wastewater achieve 3050 mL and 2150 mL in the fixed-bed column experiment, respectively. Therefore, MBCW600 presents remarkable adsorption capability, excellent recoverability and large throughput, which shows the potential application in future treatment of wastewater containing heavy metal.
引用
收藏
页数:8
相关论文
共 38 条
[1]   Valorisation possibilities of exhausted biosorbents loaded with metal ions - A review [J].
Badescu, Iulia Simona ;
Bulgariu, Dumitru ;
Ahmad, Iftikhar ;
Bulgariu, Laura .
JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2018, 224 :288-297
[2]  
Cheng S., J CLEAN PROD, V280
[3]   Potential mechanisms of cadmium removal from aqueous solution by Canna indica derived biochar [J].
Cui, Xiaoqiang ;
Fang, Siyu ;
Yao, Yiqiang ;
Li, Tingqiang ;
Ni, Qijun ;
Yang, Xiaoe ;
He, Zhenli .
SCIENCE OF THE TOTAL ENVIRONMENT, 2016, 562 :517-525
[4]   Competitive adsorption of Pb(II), Cd(II) and Cu(II) onto chitosan-pyromellitic dianhydride modified biochar [J].
Deng, Jiaqin ;
Liu, Yunguo ;
Liu, Shaobo ;
Zeng, Guangming ;
Tan, Xiaofei ;
Huang, Binyan ;
Tang, Xiaojun ;
Wang, Shengfan ;
Hua, Quan ;
Yan, Zhili .
JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2017, 506 :355-364
[5]   Simultaneous adsorption of Cr(VI) and phenol by biochar-based iron oxide composites in water: Performance, kinetics and mechanism [J].
Dong, Fu-Xin ;
Yan, Liu ;
Zhou, Xin-Hua ;
Huang, Shi-Ting ;
Liang, Jing-Yi ;
Zhang, Wen-Xuan ;
Guo, Zi-Wei ;
Guo, Peng-Ran ;
Qian, Wei ;
Kong, Ling-Jun ;
Chu, Wei ;
Diao, Zeng-Hui .
JOURNAL OF HAZARDOUS MATERIALS, 2021, 416
[6]   Valorization of biomass waste to engineered activated biochar by microwave pyrolysis: Progress, challenges, and future directions [J].
Foong, Shin Ying ;
Liew, Rock Keey ;
Yang, Yafeng ;
Cheng, Yoke Wang ;
Yek, Peter Nai Yuh ;
Mahari, Wan Adibah Wan ;
Lee, Xie Yi ;
Han, Chai Sean ;
Vo, Dai-Viet N. ;
Quyet Van Le ;
Aghbashlo, Mortaza ;
Tabatabaei, Meisam ;
Sonne, Christian ;
Peng, Wanxi ;
Lam, Su Shiung .
CHEMICAL ENGINEERING JOURNAL, 2020, 389
[7]   KOH-activated high surface area Douglas Fir biochar for adsorbing aqueous Cr(VI), Pb(II) and Cd(II) [J].
Herath, Amali ;
Layne, Cody A. ;
Perez, Felio ;
Hassan, Ei Barbary ;
Pittman, Charles U., Jr. ;
Mlsna, Todd E. .
CHEMOSPHERE, 2021, 269
[8]   Lead removal from aqueous solutions by raw sawdust and magnesium pretreated biochar: Experimental investigations and numerical modelling [J].
Jellali, Salah ;
Diamantopoulos, Efstathios ;
Haddad, Khouloud ;
Anane, Makram ;
Durner, Wolfgang ;
Mlayah, Ammar .
JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2016, 180 :439-449
[9]   A novel magnetic biochar/MgFe-layered double hydroxides composite removing Pb2+ from aqueous solution: Isotherms, kinetics and thermodynamics [J].
Jia, Yang ;
Zhang, Yingshuang ;
Fu, Jiangang ;
Yuan, Liangxiao ;
Li, Zheng ;
Liu, Chang ;
Zhao, Di ;
Wang, Xiaobo .
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS, 2019, 567 :278-287
[10]  
Kaur M., J HAZARD MATER, V417