Low-dimensional material supported single-atom catalysts for electrochemical CO2 reduction

被引：70

作者：

Wang, Bingqing ^{[1
]}

Chen, Shenghua ^{[1
]}

Zhang, Zedong ^{[1
]}

Wang, Dingsheng ^{[1
]}

机构：

[1] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China

来源：

SMARTMAT | 2022年 / 3卷 / 01期

基金：

中国国家自然科学基金; 国家重点研发计划; 中国博士后科学基金;

关键词：

ECR; electrochemical CO2 reduction; low-dimensional material; single-atom catalysts; ACTIVE-SITES; EFFICIENT ELECTROREDUCTION; ORGANIC FRAMEWORKS; CARBON; CONVERSION; FORMATE; SENSITIVITY; IRON; CU;

D O I：

10.1002/smm2.1101

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Converting CO2 emissions to valuable carbonaceous chemicals/fuels under mild conditions provides a sustainable way to maintain carbon balance and alleviate the energy shortage. Low-dimensional material (LDM) supported single-atom catalysts (SACs) have been attracted significant attention for electrochemical CO2 reduction reaction (ECR) in recent years. This is mainly because integrating the single-atoms and LDMs can inherit the advantages of themselves and the synergy effects between them are potential to enhance the ECR performance. In this review, we summarized the strategies for synthesizing LDM supported SACs for ECR, and different LDM supported SACs for ECR have been briefly introduced. Moreover, some optimization strategies for LDM supported SACs towards CO2 electroreduction are highlighted. At the end of this review, the perspectives and challenges of LDM supported SACs for ECR are provided.

引用

页码：84 / 110

页数：27

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