Polycyclic and organochlorine hydrocarbons in sediments of the northern South China Sea

被引:13
作者
Kaiser, David [1 ]
Schulz-Bull, Detlef E. [1 ]
Waniek, Joanna J. [1 ]
机构
[1] Leibniz Inst Balt Sea Res Warnemunde, D-18119 Rostock, Germany
关键词
Organic pollution; Source appointment; Sediment; South China Sea; PEARL RIVER DELTA; POLYCHLORINATED BIPHENYL CONGENERS; PERSISTENT ORGANIC POLLUTANTS; ECOLOGICAL RISK-ASSESSMENT; AROMATIC-HYDROCARBONS; SURFACE SEDIMENTS; SOURCE APPORTIONMENT; ESTUARINE SEDIMENTS; PESTICIDE-RESIDUES; EMISSION INVENTORY;
D O I
10.1016/j.marpolbul.2018.10.039
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
We investigated the concentration distribution and composition of organic pollutants in sediments of the shelf and the deep northern South China Sea (NSCS). Concentrations of polycyclic aromatic hydrocarbons (Sigma(15)PAH; 10.69-66.45 ng g(-1)), Dichlorodiphenyltrichloroethane (Sigma 4DDT; 0-0.82 ng g(-1)), and polychlorinated biphenyls (Sigma 24PCB; 0-0.12 ng g(-1)) are below established sediment quality guidelines, suggesting no environmental risk. Surprisingly, concentrations increase from the shelf to the deep NSCS, and are higher in the east of the study area. The organic pollutant composition indicates PAH mainly derived from pyrogenic sources, and mostly degraded DDT and PCB. However, in the deep NSCS, considerable contribution of petrogenic PAH, low chlorinated PCB and p,p'-DDT suggest more recent input from different sources compared to the shelf. From these results we infer that organic pollution in the NSCS does not originate from the Pearl River Estuary but from the NE SCS, SW of Taiwan.
引用
收藏
页码:668 / 676
页数:9
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