Micro-Brillouin Scattering of Relaxor Ferroelectrics with Perovskite Structure

被引:29
作者
Kojima, Seiji [1 ]
Tsukada, Shinya [1 ]
机构
[1] Grad Sch Pure & Appl Sci, Tsukuba, Ibaraki 3058573, Japan
关键词
Brillouin scattering; relaxor; polar nanoregion; random fields; TEMPERATURE-DEPENDENCE; RELAXATION; BATIO3;
D O I
10.1080/00150193.2010.482885
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Hypersonic elastic anomalies are investigated in ferroelectrics with perovskite structure by micro-Brillouin scattering to make clear the role of polar nanoregions (PNRs) and static random fields. In order to clarify the role of dynamic PNRs, the nearly second order normal ferroelectric phase transition is studied in 12 mol% KF substituted BaTiO3 (KF-BT/0.12). The precursor elastic behaviors and the critical slowing down are clearly observed above the Curie temperature TC. While in relaxor ferroelectric 0.93Pb(Zn1/3Nb2/3)O3-0.07PbTiO3 (PZN-0.07PT) with PNRs and static random fields, below the intermediate characteristic temperature T*, the suppression of slowing down of relaxation time is observed. The equation of stretched slowing down well reproduces the observed temperature dependence above TC. The growth of the characteristic localized length of dynamic PNRs is estimated as a function of temperature.
引用
收藏
页码:32 / 38
页数:7
相关论文
共 24 条
  • [1] Ferroelectric and piezoelectric properties of single crystals of Ba1-xKxTiO3-xFx with x=0.1
    Akishige, Yukikuni
    [J]. JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2006, 75 (07)
  • [2] Phase Diagram of KF-Doped BaTiO3 Single Crystals
    Akishige, Yukikuni
    [J]. FERROELECTRICS, 2008, 369 : 91 - 97
  • [3] FERROELECTRICS WITH A GLASSY POLARIZATION PHASE
    BURNS, G
    DACOL, FH
    [J]. FERROELECTRICS, 1990, 104 : 25 - 35
  • [4] THE INDEX OF REFRACTION OF BATIO3 ABOVE TC
    BURNS, G
    DACOL, FH
    [J]. FERROELECTRICS, 1981, 37 (1-4) : 661 - 664
  • [5] Precursor effects, broken local symmetry, and coexistence of order-disorder and displacive dynamics in perovskite ferroelectrics
    Bussmann-Holder, A.
    Beige, H.
    Voelkel, G.
    [J]. PHYSICAL REVIEW B, 2009, 79 (18):
  • [6] CROSS LE, 1987, FERROELECTRICS, V76, P241, DOI 10.2109/jcersj.99.829
  • [7] Intermediate temperature scale T* in lead-based relaxor systems
    Dkhil, B.
    Gemeiner, P.
    Al-Barakaty, A.
    Bellaiche, L.
    Dul'kin, E.
    Mojaev, E.
    Roth, M.
    [J]. PHYSICAL REVIEW B, 2009, 80 (06):
  • [8] RELAXATION PROCESSES IN SUPERCOOLED LIQUIDS
    GOTZE, W
    SJOGREN, L
    [J]. REPORTS ON PROGRESS IN PHYSICS, 1992, 55 (03) : 241 - 376
  • [9] Ferroelectric phase transition of stoichiometric lithium tantalate studied by Raman, Brillouin, and neutron scattering
    Hushur, Anwar
    Gvasaliya, Severian
    Roessli, Bertrand
    Lushnikov, Sergey
    Kojima, Seiji
    [J]. PHYSICAL REVIEW B, 2007, 76 (06)
  • [10] Raman scattering on the B-site order controlled by A-site substitution in relaxor Perovskite ferroelectrics
    Jiang, FM
    Kojima, S
    Zhao, CL
    Feng, CD
    [J]. JOURNAL OF APPLIED PHYSICS, 2000, 88 (06) : 3608 - 3612