Spatially Confined Hybridization of Nanometer-Sized NiFe Hydroxides into Nitrogen-Doped Graphene Frameworks Leading to Superior Oxygen Evolution Reactivity

被引:24
作者
Tang, Cheng [1 ]
Wang, Han-Sen [1 ]
Wang, Hao-Fan [1 ]
Zhang, Qiang [1 ]
Tian, Gui-Li [1 ]
Nie, Jing-Qi [1 ]
Wei, Fei [1 ]
机构
[1] Tsinghua Univ, Dept Chem Engn, Beijing Key Lab Green Chem React Engn & Technol, Beijing 100084, Peoples R China
关键词
transition metal hydroxides; graphene; catalysts; oxygen evolution; layered double hydroxides; LAYERED DOUBLE-HYDROXIDE; WATER OXIDATION; HIGH-PERFORMANCE; EFFICIENT ELECTROCATALYST; ACTIVITY ENHANCEMENT; FACILE SYNTHESIS; IN-SITU; FILM; CATALYSTS; HYBRID;
D O I
10.1002/adma.201501901
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Nanometer-sized hydroxide active centers are uniformly and strongly hybridized into a graphene framework by means of defect-anchored nucleation and spatially confined growth, resulting in a superior electrocatalyst for oxygen evolution reaction. This family of strongly coupled complexes and the topology-assisted fabrication strategy is expected to open up new avenues of research. It sheds light on a novel branch of advanced nano-architectured materials.
引用
收藏
页码:4516 / 4522
页数:7
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