Preparation and thermoelectric properties of heavily Nb-doped SrO(SrTiO3)1 epitaxial films

被引:20
作者
Lee, Kyu Hyoung
Ishizaki, Akihiro
Kim, Sung Wng
Ohta, Hiromichi
Koumoto, Kunihito [1 ]
机构
[1] Nagoya Univ, Grad Sch Engn, Nagoya, Aichi 4648603, Japan
[2] CREST, Japan Sci & Technol Agcy, Kawaguchi 3320012, Japan
[3] CREST, Japan Sci & Technol Agcy, Kawaguchi 3320012, Japan
[4] Tokyo Inst Technol, Frontier Collaborat Res Ctr, Yokohama, Kanagawa 2268503, Japan
关键词
D O I
10.1063/1.2764221
中图分类号
O59 [应用物理学];
学科分类号
摘要
We report the epitaxial film growth, by pulsed laser deposition, of c-axis-oriented Nb-doped SrO(SrTiO3)(1) films having a K2NiF4-type structure and their thermoelectric properties over a wide temperature range, from 20 to 800 K. High-resolution x-ray diffraction and reflection high energy electron diffraction patterns revealed that the films were grown heteroepitaxially on the (001) face of the LaAlO3 substrate. The thermoelectric properties of the Nb-doped SrO(SrTiO3)(1) epitaxial films were improved in terms of power factor compared to those for polycrystalline Nb-doped SrO(SrTiO3)(1). A theoretical analysis of the transport parameters revealed that the intrinsic transport occurred predominantly in the SrTiO3 layers. (c) 2007 American Institute of Physics.
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页数:4
相关论文
共 20 条
[1]  
Fistul V.I., 1969, HEAVILY DOPED SEMICO
[2]   Oriented growth of Srn+1TinO3n+1 Ruddlesden-Popper phases in chemical solution deposited thin films [J].
Gutmann, Emanuel ;
Levin, Alexandr A. ;
Reibold, Marianne ;
Mueller, Jan ;
Paufler, Peter ;
Meyer, Dirk C. .
JOURNAL OF SOLID STATE CHEMISTRY, 2006, 179 (06) :1864-1869
[3]   Epitaxial growth of the first five members of the Srn+1TinO3n+1 Ruddlesden-Popper homologous series [J].
Haeni, JH ;
Theis, CD ;
Schlom, DG ;
Tian, W ;
Pan, XQ ;
Chang, H ;
Takeuchi, I ;
Xiang, XD .
APPLIED PHYSICS LETTERS, 2001, 78 (21) :3292-3294
[4]   EFFECT OF QUANTUM-WELL STRUCTURES ON THE THERMOELECTRIC FIGURE OF MERIT [J].
HICKS, LD ;
DRESSELHAUS, MS .
PHYSICAL REVIEW B, 1993, 47 (19) :12727-12731
[5]   Artificial SrTiO3/SrO superlattices by pulsed laser deposition [J].
Iwazaki, Y ;
Suzuki, T ;
Sekiguchi, S ;
Fujimoto, M .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS, 1999, 38 (12A) :L1443-L1446
[6]   Raman spectra of carbon nanowalls grown by plasma-enhanced chemical vapor deposition [J].
Kurita, S ;
Yoshimura, A ;
Kawamoto, H ;
Uchida, T ;
Kojima, K ;
Tachibana, M ;
Molina-Morales, P ;
Nakai, H .
JOURNAL OF APPLIED PHYSICS, 2005, 97 (10)
[7]   Thermoelectric properties of layered perovskite-type (Sr1-xCax)3(Ti1-yNby)2O7 [J].
Lee, Kyu Hyoung ;
Kim, Sung Wng ;
Ohta, Hiromichi ;
Koumoto, Kunihito .
JOURNAL OF APPLIED PHYSICS, 2007, 101 (08)
[8]   Ruddlesden-Popper phases as thermoelectric oxides:: Nb-doped SrO(SrTiO3)n (n=1,2) [J].
Lee, Kyu Hyoung ;
Kim, Sung Wng ;
Ohta, Hiromichi ;
Koumoto, Kunihito .
JOURNAL OF APPLIED PHYSICS, 2006, 100 (06)
[9]  
LEVIN EM, 1969, PHASE DIAGRAMS CERAM, P93
[10]   OPTICAL ABSORPTION OF SINGLE-CRYSTAL STRONTIUM TITANATE [J].
NOLAND, JA .
PHYSICAL REVIEW, 1954, 94 (03) :724-724