Synthesis, structure and dielectric properties of zirconium and titanium oxide-doped lead oxide nano-crystalline films fabricated by sol-gel techniques for energy-storage application

被引:5
作者
Ibrahim, F. A. [1 ,2 ]
El-Desoky, M. M. [3 ]
机构
[1] Al Arish Univ, Dept Phys, Fac Sci, Al Arish, Egypt
[2] Acad Sci Res & Technol Arab Republ Egypt, Cairo, Egypt
[3] Suez Univ, Dept Phys, Fac Sci, Suez, Egypt
关键词
PBZRO3; THIN-FILMS; ELECTRICAL-PROPERTIES; PERFORMANCE; STABILITY; CERAMICS; FIELD;
D O I
10.1007/s10854-021-06500-6
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
This work aimed to improve the energy storage properties of lead zirconate (PZ) thin films by doping titanium content. Thin films of Pb-(0.9)-Zr-(0.1) (PZ) and Pb-(0.9)-(Zr-0.05.Ti-0.05)O-2 (PZT) were grown epitaxially on a glass substrate by a sol-gel colloidal route at low temperature. The structure of the obtained nanocrystals was checked by X-ray diffraction (XRD), transmission electron microscope (TEM), and electron diffraction (ED). Nanocrystals were distributed evenly of 7 +/- 0.2 for PZ and 7.5 +/- 0.2 for PZT nm in size and were closely packed. The frequency dependence of dielectric properties and the ferroelectric characteristics were detected. The energy-storage density and energy-storage efficiency estimated from hysteresis loops were about 35.15 J/cm(3) and 65.8% for (PZ) and 68.25 J/cm(3) and 66.6%for (PZT) for one layer, respectively. Results showed that the titanium content had a clear effect on the dielectric properties, ferroelectric properties, and structural properties, and on the other hand, (PZ) and (PZT) thin films had a potential application in the energy-storage device.
引用
收藏
页码:19754 / 19763
页数:10
相关论文
共 38 条
[1]  
[Anonymous], 2007, TOPICS APPL PHYS, P105
[2]   Impact of Sr-doping on structural and electrical properties of Pb(Zr0.52Ti0.48)O3 thin films on RuO2 electrodes [J].
Bag, Sankar Prasad ;
Her, Jim-Long ;
Pan, Tung-Ming .
CERAMICS INTERNATIONAL, 2017, 43 (13) :9806-9814
[3]   Effect of excess lead on the structural and electrical characteristics of sol-gel synthesized RuO2/Pb(ZrxTi1-x)O3/RuO2 [J].
Bag, Sankar Prasad ;
Her, Jim-Long ;
Pan, Tung-Ming .
CERAMICS INTERNATIONAL, 2016, 42 (16) :18402-18410
[4]   Improved energy storage properties of PbZrO3 thin films by inserting 0.88BaTiO3-0.12Bi(Mg1/2,Ti112)O3 layer [J].
Chen, T. ;
Wang, J. B. ;
Zhong, X. L. ;
Zeng, Y. K. ;
Wang, F. ;
Zhou, Y. C. .
APPLIED SURFACE SCIENCE, 2013, 285 :744-747
[5]   Superior energy-storage properties in (Pb,La)(Zr,Sn,Ti)O3 antiferroelectric ceramics with appropriate La content [J].
Dan, Yu ;
Zou, Kailun ;
Chen, Guang ;
Yu, Yuxi ;
Zhang, Ying ;
Zhang, Qingfeng ;
Lu, Yinmei ;
Zhang, Qi ;
He, Yunbin .
CERAMICS INTERNATIONAL, 2019, 45 (09) :11375-11381
[6]   Effect of residual stress on energy storage property in PbZrO3 antiferroelectric thin films with different orientations [J].
Ge, Jun ;
Remiens, Denis ;
Costecalde, Jean ;
Chen, Ying ;
Dong, Xianlin ;
Wang, Genshui .
APPLIED PHYSICS LETTERS, 2013, 103 (16)
[7]   Energy Storage Performance of Sandwich Structured Pb(Zr0.4Ti0.6)O3/BaZr0.2Ti0.8O3/Pb(Zr0.4Ti0.6)O3 Films [J].
Gu, Jinxin ;
Sun, Qiu ;
Chen, Xiangqun ;
Song, Ying ;
Tang, YiLun ;
Wang, Dongbo ;
Qu, Ping .
CRYSTALS, 2019, 9 (11)
[8]   The electrical properties and phase transformation of PLZST 2/85/13/2 antiferroelectric thin films on different bottom electrode [J].
Hao, Xihong ;
Zhai, Jiwei ;
Chou, Xiujian ;
Yao, Xi .
SOLID STATE COMMUNICATIONS, 2007, 142 (09) :498-503
[9]   A comprehensive review on the progress of lead zirconate-based antiferroelectric materials [J].
Hao, Xihong ;
Zhai, Jiwei ;
Kong, Ling Bing ;
Xu, Zhengkui .
PROGRESS IN MATERIALS SCIENCE, 2014, 63 :1-57
[10]   Composition-dependent dielectric and energy-storage properties of (Pb,La)(Zr,Sn,Ti)O3 antiferroelectric thick films [J].
Hao, Xihong ;
Wang, Ying ;
Zhang, Le ;
Zhang, Liwen ;
An, Shengli .
APPLIED PHYSICS LETTERS, 2013, 102 (16)