Effect of BiAlO3 modification on the stability of antiferroelectric phase in PbZrO3 ceramics prepared by conventional solid state reaction

被引：34
作者：
Vittayakorn, Naratip [1 ,2 ,3 ]
Boonchom, Banjong [4 ]
机构：
[1] King Mongkuts Inst Technol Ladkrabang, Dept Chem, Fac Sci, Bangkok 10520, Thailand
[2] King Mongkuts Inst Technol Ladkrabang, Coll KMITL Nanotechnol, Bangkok 10520, Thailand
[3] CHE, Thailand Ctr Excellence Phys ThEP, Bangkok 10400, Thailand
[4] King Mongkuts Inst Technol Ladkrabang, Chumphon 86160, Thailand
来源：
JOURNAL OF ALLOYS AND COMPOUNDS | 2011年 / 509卷 / 05期
关键词：
Energy storage materials; Ferroelectrics; X-ray diffraction; Dielectric response; DIELECTRIC-PROPERTIES; THERMAL-PROPERTIES; LEAD ZIRCONATE; TRANSITION; PEROVSKITE; STABILIZATION; DIFFRACTION; REFINEMENT; BOUNDARY; KINETICS;
D O I：
10.1016/j.jallcom.2010.10.206
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
In this paper, we report on the polycrystalline (Pb(1-3x/2)Bix)(Zr1-3x/4Alx)O-3 (PZO-BAO) ceramics, with x= 0.0-0.3, prepared by conventional solid state reaction. The crystal structure and thermal and dielectric properties of the sintered ceramics were investigated as a function of composition by means of X-ray diffraction (XRD), differential scanning calorimetry (DSC) and dielectric spectroscopy. The results indicated that the presence of BiAlO3: BAO in the solid solution decreased the structural stability of the overall perovskite phase. Dielectric, thermal and P-E hysteresis results confirmed that no ferroelectric intermediate phase was seen in the PZO-BAO system. An antiferroelectric phase can be stable in a wide temperature range, indicating that BAO enhanced antiferroelectric phase stability in perovskite PZ manifests by "square" antiferroelectric behavior. Therefore, the (Pb(1-3x/2)Bix)(Zr1-3x/4Alx)O-3 solid solution offers a material system for high-energy-storage capacitors and electromechanical transducers. (C) 2010 Elsevier B.V. All rights reserved.
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页码：2304 / 2310
页数：7
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