Synthesis and characterization of Pd supported on methane diamine (propyl silane) functionalized Fe3O4 nanoparticles as a magnetic catalyst for synthesis of α-aminonitriles and 2-methoxy-2-phenylacetonitrile derivative via Strecker-type reaction under ambient and solvent-free conditions

被引：3

作者：

Sun, Mingzhe ^{[1
]}

Liu, Wei ^{[2
]}

Wu, Wei ^{[1
]}

Li, Qun ^{[1
]}

Song, Di ^{[1
]}

Yan, Li ^{[3
]}

Mohammadnia, Majid ^{[4
]}

机构：

[1] Changchun Polytech, Coll Food & Biol, Changchun, Jilin, Peoples R China

[2] Jilin Normal Univ, Coll Comp Sci, Siping, Jilin, Peoples R China

[3] Jilin Normal Univ, Coll Chem, Siping 136000, Jilin, Peoples R China

[4] Islamic Azad Univ, Dept Chem, Tehran, Iran

来源：

INORGANIC AND NANO-METAL CHEMISTRY | 2023年 / 53卷 / 08期

基金：

中国国家自然科学基金;

关键词：

Pd; magnetic; nanoparticles; alpha-aminonitriles; 2-methoxy-2-phenylacetonitrile; Strecker-type reaction; ONE-POT SYNTHESIS; HIGHLY EFFICIENT CATALYST; TRIMETHYLSILYL CYANIDE; GREEN SYNTHESIS; HETEROGENEOUS CATALYST; CARBONYL-COMPOUNDS; MILD PREPARATION; ACID CATALYST; 3-COMPONENT; AMINES;

D O I：

10.1080/24701556.2021.1977819

中图分类号：

O61 [无机化学];

学科分类号：

070301 ; 081704 ;

摘要：

Pd supported on methane diamine (propyl silane) functionalized Fe3O4 magnetic nanoparticles as an organic-inorganic hybrid heterogeneous catalyst was fabricated and characterized by FT-IR, XRD, SEM, TEM, TGA, VSM, EDX, and ICP-AES techniques. The catalytic activity of the magnetic catalyst was probed through the Strecker-type reaction for one-pot synthesis of alpha-aminonitriles and 2-methoxy-2-phenylacetonitrile derivatives under ambient and solvent-free conditions. Simple procedure, high yields, short reaction time, and the environmentally benign method are advantages of this protocol. The catalyst was readily separated using an external magnet and reusable without significant loss of its catalytic efficiency.

引用

页码：861 / 875

页数：15

共 53 条

[1] Synthesis and characterization of pyridine-4-carboxylic acid-functionalized Fe3O4 nanoparticles as a magnetic catalyst for the synthesis of tetrahydrobenzo[b]pyran derivatives under solvent-free conditions
Asghari, Sakineh
Mohammadnia, Majid
[J]. INORGANIC AND NANO-METAL CHEMISTRY, 2017, 47 (07) : 1004 - 1011
[2] Preparation and characterization of sulfamic acid pyridinium chloride-functionalized Fe3O4 nanoparticles as a novel magnetic catalyst for synthesis of novel N-coumarin-2-furanones
Asghari, Sakineh
Mohammadnia, Majid
[J]. RESEARCH ON CHEMICAL INTERMEDIATES, 2017, 43 (12) : 7193 - 7209
[3] A novel approach for the synthesis of α-aminonitriles using Mitsunobu's reagent under solvent-free conditions
Chaturvedi, Devdutt
Chaturvedi, Amit K.
Mishra, Nisha
Mishra, Virendra
[J]. TETRAHEDRON LETTERS, 2012, 53 (40) : 5398 - 5401
[4] Bismuth trichloride catalyzed synthesis of α-aminonitriles
De, SK
Gibbs, RA
[J]. TETRAHEDRON LETTERS, 2004, 45 (40) : 7407 - +
[5] FERROMAGNETIC PARTICLES AS CONTRAST AGENTS FOR MAGNETIC-RESONANCE-IMAGING OF LIVER AND SPLEEN
DIAS, MHM
LAUTERBUR, PC
[J]. MAGNETIC RESONANCE IN MEDICINE, 1986, 3 (02) : 328 - 330
[6] RECENT DEVELOPMENTS IN THE STEREOSELECTIVE SYNTHESIS OF ALPHA-AMINO-ACIDS
DUTHALER, RO
[J]. TETRAHEDRON, 1994, 50 (06) : 1539 - 1650
[7] DESIGN, SYNTHESIS, AND PHARMACOLOGICAL EVALUATION OF ULTRASHORT-ACTING TO LONG-ACTING OPIOID ANALGESICS
FELDMAN, PL
JAMES, MK
BRACKEEN, MF
BILOTTA, JM
SCHUSTER, SV
LAHEY, AP
LUTZ, MW
JOHNSON, MR
LEIGHTON, HJ
[J]. JOURNAL OF MEDICINAL CHEMISTRY, 1991, 34 (07) : 2202 - 2208
[8] [HP(HNCH2CH2)3N]NO3:: an efficient homogeneous and solid-supported promoter for aza and thia-Michael reactions and for Strecker reactions
Fetterly, BA
Jana, NK
Verkade, JG
[J]. TETRAHEDRON, 2006, 62 (2-3) : 440 - 456
[9] Nano magnetic sulfated zirconia (Fe3O4@ZrO2/SO42-): an efficient solid acid catalyst for the green synthesis of α-aminonitriles and imines
Ghafuri, Hossein
Rashidizadeh, Afsaneh
Ghorbani, Behnaz
Talebi, Majid
[J]. NEW JOURNAL OF CHEMISTRY, 2015, 39 (06) : 4821 - 4829
[10] FeCl3: Highly Efficient Catalyst for Synthesis of α-Amino Nitriles
Heravi, Majid M.
Ebrahimzadeh, Mojgan
Oskooie, Hossein A.
Baghernejad, Bita
[J]. CHINESE JOURNAL OF CHEMISTRY, 2010, 28 (03) : 480 - 482

← 1 2 3 4 5 6 →