Aggregate risk assessment of polycyclic aromatic hydrocarbons from dust in an urban human settlement environment

被引:21
作者
Xu, Linyu [1 ]
Shu, Xin [1 ]
Hollert, Henner [2 ,3 ,4 ]
机构
[1] Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, 19 Xinjiekouwai St, Beijing 100875, Peoples R China
[2] Rhein Westfal TH Aachen, Dept Ecosyst Anal, Inst Environm Res Biol 5, D-52074 Aachen, Germany
[3] Chongqing Univ, Coll Resources & Environm Sci, 174 Shazhengjie, Chongqing 400044, Peoples R China
[4] Nanjing Univ, Sch Environm, 163 Xianlin Ave, Nanjing 210023, Jiangsu, Peoples R China
基金
中国国家自然科学基金;
关键词
Aggregate risk; PAHs; CLEA model; Human settlement environment; Nanjing; HEAVY-METALS; HUMAN EXPOSURE; AIR-POLLUTION; CANCER-RISK; ROAD DUST; CHINA; PAHS; DEPOSITION; CITY;
D O I
10.1016/j.jclepro.2016.05.177
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Due to the coal-dominated energy structure and increasing numbers of vehicles, gaseous polycyclic aromatic hydrocarbons (PAHs) emissions are increasing in many cities in China. These emissions have the potential to threaten human health, especially when aggregated in human settlement environments located in areas of rapid industrialization and urbanization. In this paper, an urban aggregating health risk assessment framework based on a multiple-pathways exposure model, dose risk relationships and scenario analysis, using dust as an environmental medium is proposed and examined for future study. In a case study of Nanjing, several dust samples were collected from different functional areas and the aggregate risk of polycyclic aromatic hydrocarbons in each sampling unit was assessed. The results indicated that non-carcinogenic risk and carcinogenic risk in Nanjing are currently acceptable, but cannot be ignored in the long term. The carcinogenic risk in the west of Nanjing was relatively high, but still acceptable, while it was lower in central and southeast Nanjing and lowest in the northeast. These results can be further utilized for urban planning. Future urban construction in Nanjing, especially residential construction, should be expanded to the south of the city rather than the west, to minimize the human health risk caused by industries. (C) 2016 Elsevier Ltd. All rights reserved.
引用
收藏
页码:378 / 388
页数:11
相关论文
共 40 条
[1]   Single particle characterization of size-fractionated road sediments [J].
Adachi, K ;
Tainosho, Y .
APPLIED GEOCHEMISTRY, 2005, 20 (05) :849-859
[2]  
[Anonymous], ENV SCI MANAG
[3]  
[Anonymous], 1993, EPA600R93089 OFF RES
[4]   Sources of heavy metals and polycyclic aromatic hydrocarbons in urban stormwater runoff [J].
Brown, JN ;
Peake, BM .
SCIENCE OF THE TOTAL ENVIRONMENT, 2006, 359 (1-3) :145-155
[5]  
DEFRA (Department for Environment Food and Rural Affairs), 2002, CONT LAND EXP ASS CL
[6]  
Degirmenci E, 2000, ENVIRON TOXICOL, V15, P504, DOI 10.1002/1522-7278(2000)15:5<504::AID-TOX20>3.0.CO
[7]  
2-#
[8]  
Department of the Environment Food and Rural Affairs, 2004, 11 DEP ENV ENV AG
[9]  
Department of the Environment Food and Rural Affairs, 2009, SC050021SR3 DEP ENV
[10]   Human exposure modelling for chemical risk assessment: a review of current approaches and research and policy implications [J].
Fryer, M ;
Collins, CD ;
Ferrier, H ;
Colvile, RN ;
Nieuwenhuijsen, MJ .
ENVIRONMENTAL SCIENCE & POLICY, 2006, 9 (03) :261-274