Synergistic oxidation - filtration process analysis of catalytic CuFe2O4 - Tailored ceramic membrane filtration via peroxymonosulfate activation for humic acid treatment

被引：141
作者：
Zhao, Yumeng [1 ]
Lu, Dongwei [1 ]
Xu, Chengbiao [1 ]
Zhong, Jinying [1 ]
Chen, Mansheng [1 ]
Xu, Shu [1 ]
Cao, Ying [1 ]
Zhao, Qi [1 ]
Yang, Mo [1 ]
Ma, Jun [1 ]
机构：
[1] Harbin Inst Technol, State Key Lab Urban Water Resource & Environm, Harbin 150090, Peoples R China
来源：
WATER RESEARCH | 2020年 / 171卷
基金：
中国国家自然科学基金; 中国博士后科学基金;
关键词：
Ceramic membrane; Catalytic filtration; Peroxymonosulfate oxidation; Humic acid; XDLVO theory; NATURAL ORGANIC-MATTER; DRINKING-WATER TREATMENT; ULTRAFILTRATION MEMBRANE; FULVIC-ACID; NANOFIBROUS MEMBRANES; COPPER FERRITE; DEGRADATION; FLUORESCENCE; EFFICIENT; OZONATION;
D O I：
10.1016/j.watres.2019.115387
中图分类号：
X [环境科学、安全科学];
学科分类号：
08 ; 0830 ;
摘要：
This work synthesized catalytic CuFe2O4 tailored ceramic membrane (CuFeCM), and systematically investigated the intercorrelated oxidation - filtration mechanism of peroxymonosulfate (PMS)/CuFeCM catalytic filtration for treating humic acid (HA). PMS/CuFeCM filtration exhibited enhanced HA removal efficiency while reduced the irreversible fouling resistance as compared with the conventional CM filtration. Results from HA characterizations showed that PMS/CuFeCM catalytic filtration oxidized HA into conjugated structures of smaller molecular weight. The unsaturated bonds further caused the reagglomeration of HA, hence enhancing the size exclusion of CuFeCM. Meanwhile, oxidized HA particles with changing physicochemical properties reduced the total attractive interaction energy between CuFeCM and HA, mainly attributed to the reduced acid-base interaction energy according to the Extended Derjaguin-Landau-Verwey-Overbeek (XDLVO) analysis. The changing of HA properties and HA-CuFeCM physicochemical interactions rendered more re-agglomerated HA particles retained above membrane with less attachment, which induced decreasing irreversible fouling resistance and facilitated easier external fouling removal by hydraulic cleaning. Overall, the PMS/CuFeCM configuration demonstrated in this study could provide a new insight into the synergistic oxidation - filtration interaction mechanism of hybrid catalytic ceramic membrane filtration process. (C) 2019 Elsevier Ltd. All rights reserved.
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页数：13
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共 66 条
[1]   Natural organic matter-cations complexation and its impact on water treatment: A critical review [J].
Adusei-Gyamfi, Junias ;
Ouddane, Baghdad ;
Rietveld, Luuk ;
Cornard, Jean-Paul ;
Criquet, Justine .
WATER RESEARCH, 2019, 160 :130-147
[2]   Template Assisted Microwave Synthesis of rGO-ZrO2 Composites: Efficient Photocatalysts Under Visible Light [J].
Ali, Tarek T. ;
Narasimharao, Katabathini ;
Basahel, Sulaiman N. ;
Mokhtar, Mohamed ;
Alsharaeh, Edreese H. ;
Mahmoud, Hatem A. .
JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY, 2019, 19 (08) :5177-5188
[3]   Study of the influence of graphite content on polysulfone-graphite composite membrane properties [J].
Anadao, P. ;
Sato, L. F. ;
Wiebeck, H. .
JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY, 2018, 134 (03) :1647-1656
[4]   Effects of exposure to water and ethanol on silicalite-1 membranes [J].
Andersson, Charlotte ;
Hedlund, Jonas .
JOURNAL OF MEMBRANE SCIENCE, 2008, 313 (1-2) :120-126
[5]   Urea-assisted one-step synthesis of cobalt ferrite impregnated ceramic membrane for sulfamethoxazole degradation via peroxymonosulfate activation [J].
Bao, Yueping ;
Lim, Teik-Thye ;
Wang, Rong ;
Webster, Richard David ;
Hu, Xiao .
CHEMICAL ENGINEERING JOURNAL, 2018, 343 :737-747
[6]   Mn oxide coated catalytic membranes for a hybrid ozonation-membrane filtration: Comparison of Ti, Fe and Mn oxide coated membranes for water quality [J].
Byun, S. ;
Davies, S. H. ;
Alpatova, A. L. ;
Corneal, L. M. ;
Baumann, M. J. ;
Tarabara, V. V. ;
Masten, S. J. .
WATER RESEARCH, 2011, 45 (01) :163-170
[7]   Hydraulic backwashing for low-pressure membranes in drinking water treatment: A review [J].
Chang, Haiqing ;
Liang, Heng ;
Qu, Fangshu ;
Liu, Baicang ;
Yu, Huarong ;
Du, Xing ;
Li, Guibai ;
Snyder, Shane A. .
JOURNAL OF MEMBRANE SCIENCE, 2017, 540 :362-380
[8]   Ferrous iron/peroxymonosulfate oxidation as a pretreatment for ceramic ultrafiltration membrane: Control of natural organic matter fouling and degradation of atrazine [J].
Cheng, Xiaoxiang ;
Liang, Heng ;
Ding, An ;
Tang, Xiaobin ;
Liu, Bin ;
Zhu, Xuewu ;
Gan, Zhendong ;
Wu, Daoji ;
Li, Guibai .
WATER RESEARCH, 2017, 113 :32-41
[9]   Fabrication of Mn oxide incorporated ceramic membranes for membrane fouling control and enhanced catalytic ozonation of p-chloronitrobenzene [J].
Cheng, Xiaoxiang ;
Liang, Heng ;
Qu, Fangshu ;
Ding, An ;
Chang, Haiqing ;
Liu, Bin ;
Tang, Xiaobin ;
Wu, Daoji ;
Li, Guibai .
CHEMICAL ENGINEERING JOURNAL, 2017, 308 :1010-1020
[10]   Effects of pre-ozonation on the ultrafiltration of different natural organic matter (NOM) fractions: Membrane fouling mitigation, prediction and mechanism [J].
Cheng, Xiaoxiang ;
Liang, Heng ;
Ding, An ;
Qu, Fangshu ;
Shao, Senlin ;
Liu, Bin ;
Wang, Hui ;
Wu, Daoji ;
Li, Guibai .
JOURNAL OF MEMBRANE SCIENCE, 2016, 505 :15-25
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