Environmental trade-offs of renewable jet fuels in Brazil: Beyond the carbon footprint

被引:28
作者
Capaz, Rafael S. [1 ,2 ]
de Medeiros, Elisa M. [1 ,3 ]
Falco, Daniela G. [2 ]
Seabra, Joaquim E. A. [2 ]
Osseweijer, Patricia [1 ]
Posada, John A. [1 ]
机构
[1] Delft Univ Technol TU Delft, Fac Appl Sci, Dept Biotechnol, Van der Maasweg 9, NL-2629 HZ Delft, Netherlands
[2] Univ Estadual Campinas, UNICAMP, Fac Mech Engn, R Mendeleyev 200,Cidade Univ, BR-13083860 Campinas, Brazil
[3] Univ Estadual Campinas, UNICAMP, Fac Chem Engn, Av Albert Einstein 500,Cidade Univ, BR-13083852 Campinas, Brazil
关键词
Environmental trade-offs; Life cycle assessment; Aviation biofuels; Sugarcane; Soybean; Residual feedstocks; LIFE-CYCLE ASSESSMENT; GREENHOUSE-GAS EMISSIONS; WASTE-WATER TREATMENT; ETHANOL-PRODUCTION; DIESEL; FERMENTATION; BIOFUEL;
D O I
10.1016/j.scitotenv.2020.136696
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The use of renewable jet fuels (RJFs) is an option for meeting the greenhouse gases (GHG) reduction targets of the aviation sector. Therefore, most of the studies have focused on climate change indicators, but other environmental impacts have been disregarded. In this paper, an attributional life cycle assessment is performed for ten RJF pathways in Brazil, considering the environmental trade-offs between climate change and seven other categories, i.e., fossil depletion, terrestrial acidification, eutrophication, human and environmental toxicity, and air quality-related categories, such as particulate matter and photochemical oxidant formation. The scope includes sugarcane and soybean for first-generation (1G) pathways and residual materials (wood and sugarcane residues, beef tallow, and used cooking oil-UCO) for second-generation (2G) pathways. Three certified technologies to produce RJF are considered: hydroprocessed esters and fatty acids (HEFA), alcohol-to-jet (Al)), and FischerTropsch (FT). Assuming the residual feedstocks as wastes or by-products, the 2G pathways are evaluated by two different approaches, in which the biomass sourcing processes are either accounted for or not. Results show that 1G pathways lead to significant GHG reductions compared to fossil kerosene from 55% (soybean/ HEFA) to 65% (sugarcane/ATJ). However, the sugarcane-based pathway generated three-fold higher values than fossil kerosene for terrestrial acidification and air quality impacts, and seven-fold for eutrophication. In turn, soybean/HEFA caused five-fold higher levels of human toxicity. For 2G pathways, when the residual feedstock is assumed to be waste, the potential GHG emission reduction is over 74% with no relevant trade-offs. On the other hand, if the residual feedstocks are assumed as valuable by-products, tallow/HEFA becomes the worst option and pathways from sugarcane residues, even providing a GHG reduction of 67% to 94%, are related to higher impacts than soybean/HEM for terrestrial acidification and air quality. FT pathways represent the lowest impacts for all categories within both approaches, followed by UCO/HEFA. (C) 2020 Elsevier B.V. All rights reserved.
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页数:14
相关论文
共 73 条
[1]  
ANL A.N.L., 2018, GREET NET COMP MOD
[2]  
[Anonymous], 2006, ISO14040 - Environmental management - Life cycle assessment - Principles and framework
[3]  
[Anonymous], 2019, 2019 Refinement to the 2006 IPCC Guidelines for National Greenhouse Gas Inventories
[4]  
[Anonymous], 2010, Renewable Fuel Standard
[5]  
[Anonymous], REN FUEL STAND RFS2
[6]  
[Anonymous], 2011, TECHNOECONOMIC ENV A
[7]  
[Anonymous], 2002, A comprehensive analysis of biodiesel impacts on exhaust emissions
[8]  
ANP, 2019, OIL NAT GAS BIOF STA
[9]  
Anp, 2018, REN NAT POL BIOF
[10]  
ASTM, 2019, D756619 ASTM