A 100 year sedimentary record of heavy metal pollution in a shallow eutrophic lake, Lake Chaohu, China

被引:63
作者
Zan, Fengyu [1 ,2 ]
Huo, Shouliang [1 ]
Xi, Beidou [1 ]
Su, Jing [1 ]
Li, Xiang [1 ]
Zhang, Jingtian [1 ]
Yeager, Kevin M. [3 ]
机构
[1] Chinese Res Inst Environm Sci, State Key Lab Environm Criteria & Risk Assessment, Beijing 100012, Peoples R China
[2] Anhui Normal Univ, Coll Environm Sci & Engn, Wuhu 241000, Anhui, Peoples R China
[3] Univ So Mississippi, Dept Marine Sci, Stennis Space Ctr, MS 39529 USA
来源
JOURNAL OF ENVIRONMENTAL MONITORING | 2011年 / 13卷 / 10期
基金
中国国家自然科学基金;
关键词
TRACE; RADIONUCLIDES; HEALTH; COPPER; SOILS; PB; CD; CU;
D O I
10.1039/c1em10385g
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
This study has worked on the evaluation of the temporal and spatial evolution of heavy metal contamination in sediment taken from a shallow eutrophic lake, Lake Chaohu, China, over the last 100 years, and thereby used Cs-137 and Pb-210 dating, a PIRLA procedure, statistical analysis, geochemical normalization and a enrichment factor calculation (EF). Concentrations of 5174, 29 325, 10.7, 36.4, 20.4, 386.0, 21.1 and 38.4 mg kg(-1) for Ti, Fe, Co, Cr, Cu, Mn, Pb and Zn, respectively, are proposed as natural background values for the Lake Chaohu based on a PIRLA procedure. The contamination history from the last 100 years can be divided into two periods. Before the 1960s, heavy metal contamination did not occur and there was no spatial difference for heavy metal distribution. Since the 1960s, heavy metal enrichment and contamination has occurred, and the west half of the lake region showed a higher degree of contamination than the east half to various intensified anthropogenic activities. In the east half of the lake region, the anthropogenic source of heavy metals mainly originated from agricultural intensification, whereas in the west half of the lake it originated from city runoff and industry as well as agriculture. In all anthropogenic heavy metals, Co is only from industry.
引用
收藏
页码:2788 / 2797
页数:10
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