Scratch-Healing Behavior of Ice by Local Sublimation and Condensation

被引：9

作者：

Demmenie, Menno ^{[1
,3
]}

Kolpakov, Paul ^{[1
]}

Nagata, Yuki ^{[2
]}

Woutersen, Sander ^{[3
]}

Bonn, Daniel ^{[1
]}

机构：

[1] Univ Amsterdam, Inst Phys, NL-1098 XH Amsterdam, Netherlands

[2] Max Planck Inst Polymer Res, D-55128 Mainz, Germany

[3] Univ Amsterdam, Vant Hoff Inst Mol Sci, NL-1098 XH Amsterdam, Netherlands

来源：

JOURNAL OF PHYSICAL CHEMISTRY C | 2022年 / 126卷 / 04期

关键词：

DESORPTION-KINETICS; MASS-TRANSFER; SOLAR-SYSTEM; WATER-ICE; SURFACE; DIFFUSION; MICROSTRUCTURE; EVOLUTION; MODEL;

D O I：

10.1021/acs.jpcc.1c09590

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We show that the surface of ice is scratch healing: micrometer-deep scratches in the ice surface spontaneously disappear by thermal relaxation on the time scale of roughly an hour. Following the dynamics and comparing it to different mass transfer mechanisms, we find that sublimation from and condensation onto the ice surface is the dominant scratch-healing mechanism. The scratch-healing kinetics shows a strong temperature dependence, following an Arrhenius behavior with an activation energy of Delta E = 58.6 +/- 4.6 kJ/mol, agreeing with the proposed sublimation mechanism and at odds with surface diffusion or fluid flow or evaporation-condensation from a quasi-liquid layer.

引用

页码：2179 / 2183

页数：5

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