Frenetic aspects of second order response

被引:36
作者
Basu, Urna [1 ]
Krueger, Matthias [2 ,3 ]
Lazarescu, Alexandre [1 ]
Maes, Christian [1 ]
机构
[1] Katholieke Univ Leuven, Inst Theoret Fys, Leuven, Belgium
[2] Univ Stuttgart, Inst Theoret Phys 4, D-70174 Stuttgart, Germany
[3] Max Planck Inst Intelligent Syst, Stuttgart, Germany
关键词
NONLINEAR RESPONSE;
D O I
10.1039/c4cp04977b
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Starting from the second order around thermal equilibrium, the response of a statistical mechanical system to an external stimulus is not only governed by dissipation and depends explicitly on dynamical details of the system. The so called frenetic contribution in the second order around equilibrium is illustrated in different physical examples, such as for non-thermodynamic aspects in the coupling between a system and reservoir, for the dependence on disorder in the dielectric response and for the nonlinear correction to the Sutherland-Einstein relation. More generally, the way in which a system's dynamical activity changes by perturbation is visible (only) from the nonlinear response.
引用
收藏
页码:6653 / 6666
页数:14
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