Effect of the charge balance on high-efficiency inverted polymer light-emitting diodes

被引:11
作者
Huang, Qingyu [1 ,2 ]
Zhao, Suling [1 ]
Guo, L. Jay [2 ]
Xu, Zheng [1 ]
Wang, Peng [1 ]
Qin, Zilun [1 ]
机构
[1] Beijing Jiaotong Univ, Key Lab Luminescence & Opt Informat, Minist Educ, Beijing 100044, Peoples R China
[2] Univ Michigan, Dept Elect Engn & Comp Sci, Ann Arbor, MI 48105 USA
基金
中国国家自然科学基金;
关键词
Inverted polymer light emitting devices; Charge balance; Electron injection; Hole injection; ELECTRON-INJECTION; QUANTUM DOTS; LAYER; ELECTROLUMINESCENCE; PERFORMANCE; DEVICES;
D O I
10.1016/j.orgel.2017.05.028
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
In this work, an ultra-thin insulating layer, poly(methylmethacrylate) (PMMA), is incorporated between the emissive layer (EML) and hole transporting layer (HTL) within the inverted polymer light-emitting diodes (PLEDs). Such a structure helps to reduce the hole injection and balance the electrons and holes in the EML. PLEDs with optimal PMMA thickness of around 5.6 nm is observed to obtain a maximum current efficiency of 14.33 cd A(-1), which corresponds to 7.07% improvement compared to that of the device without PMMA layer (13.5 cd A(-1)). The device with best performance exhibits a superior low driving voltage of 2.5 V at 1 cd m(-2) and shows a lower efficiency roll-off current efficiency which sustains 85% of the maximum value when the current density reaches 140 mA cm(-2). (C) 2017 Published by Elsevier B.V.
引用
收藏
页码:123 / 128
页数:6
相关论文
共 25 条
[21]   A Hybrid Inorganic-Organic Semiconductor Light-Emitting Diode Using ZrO2 as an Electron-Injection Layer [J].
Tokmoldin, Nurlan ;
Griffiths, Nicholas ;
Bradley, Donal D. C. ;
Haque, Saif A. .
ADVANCED MATERIALS, 2009, 21 (34) :3475-+
[22]   Electron transport and electroluminescent efficiency of conjugated polymers [J].
Tseng, S. R. ;
Chen, Y. S. ;
Meng, H. F. ;
Lai, H. C. ;
Yeh, C. H. ;
Horng, S. F. ;
Liao, H. H. ;
Hsu, C. S. .
SYNTHETIC METALS, 2009, 159 (1-2) :137-141
[23]   ITO-free top emitting organic light emitting diodes with enhanced light out-coupling [J].
Yambem, Soniya D. ;
Ullah, Mujeeb ;
Tandy, Kristen ;
Burn, Paul L. ;
Namdas, Ebinazar B. .
LASER & PHOTONICS REVIEWS, 2014, 8 (01) :165-171
[24]   An Ultrathin, Smooth, and Low-Loss Al-Doped Ag Film and Its Application as a Transparent Electrode in Organic Photovoltaics [J].
Zhang, Cheng ;
Zhao, Dewei ;
Gu, Deen ;
Kim, Hyunsoo ;
Ling, Tao ;
Wu, Yi-Kuei Ryan ;
Guo, L. Jay .
ADVANCED MATERIALS, 2014, 26 (32) :5696-+
[25]   A Universal Method to Produce Low-Work Function Electrodes for Organic Electronics [J].
Zhou, Yinhua ;
Fuentes-Hernandez, Canek ;
Shim, Jaewon ;
Meyer, Jens ;
Giordano, Anthony J. ;
Li, Hong ;
Winget, Paul ;
Papadopoulos, Theodoros ;
Cheun, Hyeunseok ;
Kim, Jungbae ;
Fenoll, Mathieu ;
Dindar, Amir ;
Haske, Wojciech ;
Najafabadi, Ehsan ;
Khan, Talha M. ;
Sojoudi, Hossein ;
Barlow, Stephen ;
Graham, Samuel ;
Bredas, Jean-Luc ;
Marder, Seth R. ;
Kahn, Antoine ;
Kippelen, Bernard .
SCIENCE, 2012, 336 (6079) :327-332