Theory of Half-Metallic Ferrimagnetism in Double Perovskites

被引:86
作者
Erten, Onur [1 ]
Meetei, O. Nganba [1 ]
Mukherjee, Anamitra [1 ]
Randeria, Mohit [1 ]
Trivedi, Nandini [1 ]
Woodward, Patrick [2 ]
机构
[1] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA
[2] Ohio State Univ, Dept Chem, Columbus, OH 43210 USA
基金
美国国家科学基金会;
关键词
DISORDER;
D O I
10.1103/PhysRevLett.107.257201
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Double perovskites such as Sr2FeMoO6 are rare examples of materials with half-metallic ground states and a ferrimagnetic T-c above room temperature. We present a comprehensive theory of the temperature and disorder dependence of their magnetic properties by deriving and validating a new effective spin Hamiltonian for these materials, amenable to large-scale three-dimensional simulations. We show how disorder, ubiquitous in these materials, affects T-c, the magnetization, and the conduction electron polarization. We conclude with a novel proposal to enhance T-c without sacrificing polarization.
引用
收藏
页数:4
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