Liquid-Phase Vibrational Strong Coupling

被引:148
作者
George, Jino
Shalabney, Atef
Hutchison, James A.
Genet, Cyriaque
Ebbesen, Thomas W. [1 ]
机构
[1] Univ Strasbourg, ISIS, F-67000 Strasbourg, France
关键词
LIGHT-MATTER INTERACTIONS; SURFACE-PLASMON; ROOM-TEMPERATURE; VACUUM FIELD; MICROCAVITIES; NANOSTRUCTURES; ENHANCEMENT; ABSORPTION; RESONANCES; EXCITONS;
D O I
10.1021/acs.jpclett.5b00204
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Light-matter strong coupling involving ground-state molecular vibrations is investigated for the first time in the liquid phase for a set of molecules placed in microcavities. By tuning the cavities, one or more vibrational modes can be coupled in parallel or in series, inducing a change in the vibrational frequencies of the bonds. These findings are of fundamental importance to fully develop light matter strong coupling for applications in molecular and material sciences.
引用
收藏
页码:1027 / 1031
页数:5
相关论文
共 42 条
[1]   Plasmon-Exciton Interactions in a Core-Shell Geometry: From Enhanced Absorption to Strong Coupling [J].
Antosiewicz, Tomasz J. ;
Apell, S. Peter ;
Shegai, Timur .
ACS PHOTONICS, 2014, 1 (05) :454-463
[2]   Active Control of the Strong Coupling Regime between Porphyrin Excitons and Surface Plasmon Polaritons [J].
Berrier, Audrey ;
Cools, Ruud ;
Arnold, Christophe ;
Offermans, Peter ;
Crego-Calama, Mercedes ;
Brongersma, Sywert H. ;
Rivas, Jaime Gomez .
ACS NANO, 2011, 5 (08) :6226-6232
[3]   Non-Markovian polariton dynamics in organic strong coupling [J].
Canaguier-Durand, Antoine ;
Genet, Cyriaque ;
Lambrecht, Astrid ;
Ebbesen, ThomasW. ;
Reynaud, Serge .
EUROPEAN PHYSICAL JOURNAL D, 2015, 69 (01)
[4]   Thermodynamics of Molecules Strongly Coupled to the Vacuum Field [J].
Canaguier-Durand, Antoine ;
Devaux, Eloise ;
George, Jino ;
Pang, Yantao ;
Hutchison, James A. ;
Schwartz, Tal ;
Genet, Cyriaque ;
Wilhelms, Nadine ;
Lehn, Jean-Marie ;
Ebbesen, Thomas W. .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2013, 52 (40) :10533-10536
[5]   Strong coupling between surface plasmon-polaritons and organic molecules in subwavelength hole arrays [J].
Dintinger, J ;
Klein, S ;
Bustos, F ;
Barnes, WL ;
Ebbesen, TW .
PHYSICAL REVIEW B, 2005, 71 (03)
[6]   LIGHT-MATTER INTERACTIONS Ultrastrong routes to new chemistry [J].
Fontcuberta i Morral, Anna ;
Stellacci, Francesco .
NATURE MATERIALS, 2012, 11 (04) :272-273
[7]   Tunable polariton absorption of distributed feedback microcavities at room temperature [J].
Fujita, T ;
Sato, Y ;
Kuitani, T ;
Ishihara, T .
PHYSICAL REVIEW B, 1998, 57 (19) :12428-12434
[8]   Exploring Light-Matter Interaction Phenomena under Ultrastrong Coupling Regime [J].
Gambino, Salvatore ;
Mazzeo, Marco ;
Genco, Armando ;
Di Stefano, Omar ;
Savasta, Salvatore ;
Patane, Salvatore ;
Ballarini, Dario ;
Mangione, Federica ;
Lerario, Giovanni ;
Sanvitto, Daniele ;
Gigli, Giuseppe .
ACS PHOTONICS, 2014, 1 (10) :1042-1048
[9]   Semiclassical Plexcitonics: Simple Approach for Designing Plexcitonic Nanostructures [J].
Gomez, Daniel E. ;
Giessen, Harald ;
Davis, Timothy J. .
JOURNAL OF PHYSICAL CHEMISTRY C, 2014, 118 (41) :23963-23969
[10]   Picosecond Kinetics of Strongly Coupled Excitons and Surface Plasmon Polaritons [J].
Gomez, Daniel E. ;
Lo, Shun Shang ;
Davis, Timothy J. ;
Hartland, Gregory V. .
JOURNAL OF PHYSICAL CHEMISTRY B, 2013, 117 (16) :4340-4346