Spectroscopic evidence for a type II Weyl semimetallic state in MoTe2

被引:455
作者
Huang, Lunan [1 ,2 ]
McCormick, Timothy M. [3 ,4 ]
Ochi, Masayuki [5 ]
Zhao, Zhiying [6 ]
Suzuki, Michi-To [7 ]
Arita, Ryotaro [7 ,8 ]
Wu, Yun [1 ,2 ]
Mou, Daixiang [1 ,2 ]
Cao, Huibo [9 ]
Yan, Jiaqiang [10 ,11 ]
Trivedi, Nandini [3 ,4 ]
Kaminski, Adam [1 ,2 ]
机构
[1] US DOE, Ames Lab, Ames, IA 50011 USA
[2] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA
[3] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA
[4] Ohio State Univ, Ctr Emergent Mat, Columbus, OH 43210 USA
[5] Osaka Univ, Dept Phys, Toyonaka, Osaka 5600043, Japan
[6] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA
[7] RIKEN, CEMS, Wako, Saitama 3510198, Japan
[8] Tohoku Univ, JST ERATO Isobe Degenerate Integrat Project, AIMR, Sendai, Miyagi 9808577, Japan
[9] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA
[10] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA
[11] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA
基金
美国国家科学基金会;
关键词
WANNIER FUNCTIONS; FERMI ARCS; DISCOVERY; PHASE; TAAS;
D O I
10.1038/nmat4685
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In a type I Dirac or Weyl semimetal, the low-energy states are squeezed to a single point in momentum space when the chemical potential mu is tuned precisely to the Dirac/Weyl point(1-6). Recently, a type II Weyl semimetal was predicted to exist, where the Weyl states connect hole and electron bands, separated by an indirect gap(7-10). This leads to unusual energy states, where hole and electron pockets touch at the Weyl point. Here we present the discovery of a type II topological Weyl semimetal state in pure MoTe2, where two sets of Weyl points. (W2(+/-), W3(+/-)) exist at the touching points of electron and hole pockets and are located at different binding energies above E-F. Using angle-resolved photoemission spectroscopy, modelling, density functional theory and calculations of Berry curvature, we identify the Weyl points and demonstrate that they are connected by different sets of Fermi arcs for each of the two surface terminations. We also find new surface 'track states' that form closed loops and are unique to type II Weyl semimetals. This material provides an exciting, new platform to study the properties of Weyl fermions.
引用
收藏
页码:1155 / +
页数:7
相关论文
共 30 条
[1]  
Belopolski I., 2015, PREPRINT
[2]  
Blaha P., 2001, Calculating Cryst. Prop., V60
[3]   Topological nodal semimetals [J].
Burkov, A. A. ;
Hook, M. D. ;
Balents, Leon .
PHYSICAL REVIEW B, 2011, 84 (23)
[4]   Weyl Semimetal in a Topological Insulator Multilayer [J].
Burkov, A. A. ;
Balents, Leon .
PHYSICAL REVIEW LETTERS, 2011, 107 (12)
[5]   Use of frit-disc crucibles for routine and exploratory solution growth of single crystalline samples [J].
Canfield, Paul C. ;
Kong, Tai ;
Kaluarachchi, Udhara S. ;
Jo, Na Hyun .
PHILOSOPHICAL MAGAZINE, 2016, 96 (01) :84-92
[6]   Single-cell Migration Chip for Chemotaxis-based Microfluidic Selection of Heterogeneous Cell Populations [J].
Chen, Yu-Chih ;
Allen, Steven G. ;
Ingram, Patrick N. ;
Buckanovich, Ronald ;
Merajver, Sofia D. ;
Yoon, Euisik .
SCIENTIFIC REPORTS, 2015, 5
[7]   Dimensional crossover in topological matter: Evolution of the multiple Dirac point in the layered system to the flat band on the surface [J].
Heikkila, T. T. ;
Volovik, G. E. .
JETP LETTERS, 2011, 93 (02) :59-65
[8]   A topological Dirac insulator in a quantum spin Hall phase [J].
Hsieh, D. ;
Qian, D. ;
Wray, L. ;
Xia, Y. ;
Hor, Y. S. ;
Cava, R. J. ;
Hasan, M. Z. .
NATURE, 2008, 452 (7190) :970-U5
[9]   New type of Weyl semimetal with quadratic double Weyl fermions [J].
Huang, Shin-Ming ;
Xu, Su-Yang ;
Belopolski, Ilya ;
Lee, Chi-Cheng ;
Chang, Guoqing ;
Chang, Tay-Rong ;
Wang, BaoKai ;
Alidoust, Nasser ;
Bian, Guang ;
Neupane, Madhab ;
Sanchez, Daniel ;
Zheng, Hao ;
Jeng, Horng-Tay ;
Bansil, Arun ;
Neupert, Titus ;
Lin, Hsin ;
Hasan, M. Zahid .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2016, 113 (05) :1180-1185
[10]   Tunable vacuum ultraviolet laser based spectrometer for angle resolved photoemission spectroscopy [J].
Jiang, Rui ;
Mou, Daixiang ;
Wu, Yun ;
Huang, Lunan ;
McMillen, Colin D. ;
Kolis, Joseph ;
Giesber, Henry G., III ;
Egan, John J. ;
Kaminski, Adam .
REVIEW OF SCIENTIFIC INSTRUMENTS, 2014, 85 (03)