Phonon softening, chaotic motion, and order-disorder transition in Sn/Ge(111) -: art. no. 016103

被引:44
作者
Farías, D
Kaminski, W
Lobo, J
Ortega, J
Hulpke, E
Pérez, R
Flores, F
Michel, EG
机构
[1] Univ Autonoma Madrid, Dept Fis Mat Condensada, E-28049 Madrid, Spain
[2] Univ Autonoma Madrid, Inst Nicolas Cabrera, E-28049 Madrid, Spain
[3] Univ Autonoma Madrid, Dept Fis Teor Mat Condesada, E-28049 Madrid, Spain
[4] Univ Wroclaw, Inst Phys Expt, PL-50204 Wroclaw, Poland
[5] Max Planck Inst Stromungsforsch, D-37073 Gottingen, Germany
关键词
D O I
10.1103/PhysRevLett.91.016103
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The phonon dynamics of the Sn/Ge(111) interface is studied using high-resolution helium atom scattering and first-principles calculations. At room temperature we observe a phonon softening at then (K) over bar point in the (root3xroot3)R30degrees phase, associated with the stabilization of a (3x3) phase at low temperature. That phonon band is split into three branches in the (3x3) phase. We analyze the character of these phonons and find out that the low- and room-temperature modes are connected via a chaotic motion of the Sn atoms. The system is shown to present an order-disorder transition.
引用
收藏
页码:1 / 016103
页数:4
相关论文
共 23 条
[1]   Dynamical fluctuations as the origin of a surface phase transition in Sn/Ge(III) [J].
Avila, J ;
Mascaraque, A ;
Michel, EG ;
Asensio, MC ;
LeLay, G ;
Ortega, J ;
Pérez, R ;
Flores, F .
PHYSICAL REVIEW LETTERS, 1999, 82 (02) :442-445
[2]   Disproportionation phenomena on free and strained Sn/Ge(111) and Sn/Si(111) surfaces [J].
Ballabio, G ;
Profeta, G ;
de Gironcoli, S ;
Scandolo, S ;
Santoro, GE ;
Tosatti, E .
PHYSICAL REVIEW LETTERS, 2002, 89 (12) :126803-126803
[3]   √3X √3R30° versus adatom-rest-atom phases on (111) semiconductor surfaces [J].
Ballabio, G ;
Scandolo, S ;
Tosatti, E .
PHYSICAL REVIEW B, 2000, 61 (20) :13345-13348
[4]  
BENEDEK G, 1992, HELIUM ATOM SCATTERI, P195
[5]   Surface charge ordering transition: alpha phase of Sn/Ge(111) [J].
Carpinelli, JM ;
Weitering, HH ;
Bartkowiak, M ;
Stumpf, R ;
Plummer, EW .
PHYSICAL REVIEW LETTERS, 1997, 79 (15) :2859-2862
[6]   ELECTRONIC-STRUCTURE APPROACH FOR COMPLEX SILICAS [J].
DEMKOV, AA ;
ORTEGA, J ;
SANKEY, OF ;
GRUMBACH, MP .
PHYSICAL REVIEW B, 1995, 52 (03) :1618-1630
[7]   HELIUM-ATOM-SCATTERING STUDY OF THE STRUCTURE AND PHONON DYNAMICS OF THE W(001) SURFACE BETWEEN 200-K AND 1900-K [J].
ERNST, HJ ;
HULPKE, E ;
TOENNIES, JP .
PHYSICAL REVIEW B, 1992, 46 (24) :16081-16105
[8]   Helium scattering structure analyses of the c(2x8) reconstruction and the high-temperature (1x1) structures of Ge(111) [J].
Farias, D ;
Lange, G ;
Rieder, KH ;
Toennies, JP .
PHYSICAL REVIEW B, 1997, 55 (11) :7023-7033
[9]   Atomic beam diffraction from solid surfaces [J].
Farías, D ;
Rieder, KH .
REPORTS ON PROGRESS IN PHYSICS, 1998, 61 (12) :1575-1664
[10]   Order-disorder transition of the (3X3) Sn/Ge(111) phase [J].
Floreano, L ;
Cvetko, D ;
Bavdek, G ;
Benes, M ;
Morgante, A .
PHYSICAL REVIEW B, 2001, 64 (07)