Facile Synthesis of Mn doped Bi2S3 Photocatalyst for Efficient Degradation of Organic Dye under Visible-Light Irradiation

被引:47
作者
Iqbal, Muzaffar [1 ]
Ibrar, Aliya [1 ]
Ali, Ashraf [1 ]
Hussain, Shabeeb [1 ]
Shad, Salma [1 ]
Ullah, Sami [2 ]
Alshahrani, Thamraa [3 ]
Hakami, Jabir [4 ]
Khan, Firoz [5 ]
Thebo, Khalid Hussain [6 ]
机构
[1] Univ Haripur KPK, Fac Nat Sci, Dept Chem, Haripur 22620, Pakistan
[2] King Fahd Univ Petr & Minerals KFUPM, KA CARE Energy Res & Innovat Ctr ER, Dhahran 31261, Saudi Arabia
[3] Princess Nourah bint Abdulrahman Univ, Coll Sci, Dept Phys, POB 84428, Riyadh 11671, Saudi Arabia
[4] Jazan Univ, Coll Sci, Dept Phys, POB 114, Jazan 45142, Saudi Arabia
[5] King Fahd Univ Petr & Minerals KFUPM, Res Inst, Interdisciplinary Res Ctr Renewable Energy & Power, Dhahran 31261, Saudi Arabia
[6] Chinese Acad Sci, Inst Met Res IMR, Wenhua Rd, Shenyang, Peoples R China
关键词
nanoflower; hydrothermal; photocatalyst; rhodamineB; METHYLENE-BLUE; RHODAMINE-B; MICROSPHERES; NANOFLOWERS; OXIDE;
D O I
10.1016/j.molstruc.2022.133598
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The development of high performance photocatalyst with wider visible light adsorption, photo electrochemically stable and good efficient charge separation is highly desire for clean energy applications in recent days. Herein, a simple hydrothermal method is used to successfully prepare Mn doped Bi 2 S 3 nanoflowers using different dopant concentration ranging from 1% to 3%. The X-ray diffraction, scanning electron microscope, X-ray photoelectron spectroscopy, and ultra-violet spectroscopic technique were used to study the physicochemical and morphological characterization of as-prepared materials. While the charge separation and recombination processes were investigated with help of electrochemical impedance spectroscopy (EIS) and photo transient response. Further, we investigated the photodegradation studies of rhodamine B (RhB) dye under visible light illumination using Mn doped Bi 2 S 3 -based nanostructures. Results shows that the 3% Mn doped Bi 2 S 3 nanostructure exhibits superior degradation studies. Finally the photocatalysis degradation mechanism is also studied in detail. We believe, this work will open a new direction for readers to develop highly efficient photocatalysts for resolve water pollution issue.
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页数:9
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