Dynamic processes on vanadium phosphorous oxides for selective alkane oxidation

被引:57
作者
Volta, JC
机构
[1] Inst. de Recherches sur la Catalyse, CNRS, F-69626 Villeurbanne Cédex
关键词
dynamic processes; vanadium phosphorous oxides; selective alkane oxidation;
D O I
10.1016/S0920-5861(96)00073-9
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
The use of complementary physicochemical tools (XRD, Raman spectroscopy, XPS, P-31 NMR, and electron microscopy techniques), sometimes used in in situ conditions has allowed to evidence the dynamic processes occurring during the oxidation of light alkanes on the vanadium phosphorus oxide (VPO) system. The transformations of the VPO system in the course of the oxidation of n-butane to maleic anhydride and of the oxidation of propane to acrylic acid are contrasted in connection with the evolution of the catalytic performances.
引用
收藏
页码:29 / 36
页数:8
相关论文
共 18 条
  • [1] EVOLUTION OF A VPO CATALYST IN N-BUTANE OXIDATION REACTION DURING THE ACTIVATION TIME
    ABON, M
    BERE, KE
    TUEL, A
    DELICHERE, P
    [J]. JOURNAL OF CATALYSIS, 1995, 156 (01) : 28 - 36
  • [2] OXIDATION OF PROPANE TO ACRYLIC-ACID ON V2O5-P2O5-BASED CATALYSTS
    AI, M
    [J]. JOURNAL OF CATALYSIS, 1986, 101 (02) : 389 - 395
  • [3] A STUDY BY INSITU LASER RAMAN-SPECTROSCOPY OF VPO CATALYSTS FOR NORMAL-BUTANE OXIDATION TO MALEIC-ANHYDRIDE .1. PREPARATION AND CHARACTERIZATION OF PURE REFERENCE PHASES
    BENABDELOUAHAB, F
    OLIER, R
    GUILHAUME, N
    LEFEBVRE, F
    VOLTA, JC
    [J]. JOURNAL OF CATALYSIS, 1992, 134 (01) : 151 - 167
  • [4] BENABDELOUAHAB F, IN PRESS J CATAL
  • [5] Bordes E., 1987, CATAL TODAY, V1, P499, DOI DOI 10.1016/0920-5861(87)85003-4
  • [6] MECHANISTIC ASPECTS OF MALEIC-ANHYDRIDE SYNTHESIS FROM C4-HYDROCARBONS OVER PHOSPHORUS VANADIUM-OXIDE
    CENTI, G
    TRIFIRO, F
    EBNER, JR
    FRANCHETTI, VM
    [J]. CHEMICAL REVIEWS, 1988, 88 (01) : 55 - 80
  • [7] CENTI G, 1993, CATAL TODAY, V16
  • [8] COURTINE P, 1985, SOLID STATE CHEM CAT, P37
  • [9] GRASSELLI RK, 1981, SELECTIVE OXIDATION, V30
  • [10] HABER J, 1984, 8 INT C CAT BERL 198, P1