On the relation between Stokes and anti-Stokes light scattering in liquids

被引：6
|
作者：
Surovtsev, NV [1 ]
机构：
[1] Russian Acad Sci, Inst Automat & Electrometry, Lab 04, Novosibirsk 630090, Russia
来源：
CHEMICAL PHYSICS LETTERS | 2003年 / 375卷 / 5-6期
关键词：
D O I：
10.1016/S0009-2614(03)00932-1
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
The problem discussed is whether the relation between Stokes and anti-Stokes light scattering in liquids follows the famous expression I-S/I-AS = exp(hv/kT). It is demonstrated that the disagreement of this expression with the results found by Watanabe et al. [Chem. Phys. Lett. 333 (2001) 113] is related to the wrong procedure of the determination of the origin of the spectra used in this work. It is shown that in framework of the standard paradigm the relaxational mode in light-scattering spectrum of liquids is placed at a non-zero frequency about 10(-2) cm(-1) in Stokes side of spectrum. (C) 2003 Elsevier Science B.V. All rights reserved.
引用
收藏
页码：495 / 498
页数：4
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